Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 22, Issue 41, Pages 14508-14512Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201602936
Keywords
C-H functionalization; indoles; N-N bond cleavage; olefination; ruthenium
Categories
Funding
- National Natural Science Foundation of China [21425415, 21274058]
- National Basic Research Program of China [2015CB856303]
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A previously elusive Ru-II-catalyzed N-N bond-based traceless C-H functionalization strategy is reported. An N-amino (i.e., hydrazine) group is used for the directed C-H functionalization with either an alkyne or an alkene, affording an indole derivative or olefination product. The synthesis features a broad substrate scope, superior atom and step economy, as well as mild reaction conditions.
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