Journal
APPLIED SURFACE SCIENCE
Volume 509, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.apsusc.2020.145360
Keywords
Polydopamine; Janus particles; Colloidal crystals; Asymmetry; Functionality
Categories
Funding
- National Natural Science Foundation of China [51473089]
- Natural Science Basic Research Plan in Shaanxi Province of China [2018JM5093]
- Program for Science & Technology Innovation Team of Shaanxi Province [2018TD-030]
- Fundamental Research Funds for the Central Universities [GK201702009, GK201901002]
- Academy of Finland [321443, 328942]
- Academy of Finland (AKA) [328942, 328942, 321443, 321443] Funding Source: Academy of Finland (AKA)
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Janus particles with controlled asymmetries and functionalities represent promising building blocks and functional materials due to their unique anisotropic features. Herein, we show a facile and general approach towards preparing colloidal Janus particles with adjustable surface asymmetries and functionalities based on monolayer colloidal crystal (MCC) templates combined with mussel-inspired polydopamine (PDA) chemistry at an air-water interface. First, monodisperse colloidal polystyrene/polydopamine (PS/PDA) Janus particles with tunable asymmetrical geometries are synthesized by polymerizing dopamine onto two-dimensional (2D) polystyrene (PS) monolayer colloidal crystals formed at the air-water interface. Moreover, the good chemical reactivity of the PDA coating makes it a versatile platform to introduce a variety of functional materials, e.g., metal nanoparticles and organic molecules, producing colloidal Janus particles with adjustable functionalities. Finally, we demonstrate this synthetic strategy not only provides a controllable method for the fabrication of monodisperse colloidal Janus particles but also opens up a new Janus platform for artificially designed Janus particles with tunable asymmetries and functionalities.
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