Journal
PHYSICAL REVIEW APPLIED
Volume 13, Issue 2, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevApplied.13.024051
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Funding
- National Natural Science Foundation of China [61704153, 61774019]
- Zhejiang Public Service Technology Research Program/Analytical Test [LGC19F040001]
- Natural Science Foundation of Zhejiang Province [LY20F040005]
- Visiting Scholar Foundation of State Key Lab of Silicon Materials [SKL2019-08]
- Fundamental Research Funds of Zhejiang Sci-Tech University [2019Q061, 2019Q067]
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Self-powered Ga2O3-based solar-blind photodetectors have received attention recently due to the increased demand for energy saving, miniaturization, and high efficiency in devices. An ideal device structure consisting of a Ga2O3-based p-n junction is still difficult to obtain, since p-type doping is a major challenge. Although self-powered devices based on heterojunction are promising, there are two fatal disadvantages: (1) photosensitivity of the non-solar-blind region, on account of the narrower band gap of the heterojunction materials; and (2) poor quality of the epitaxial film due to lattice mismatch. In view of the various polymorphs of Ga2O3, we propose constructing a structure consisting of a Ga2O3 phase junction with alpha and beta phases (alpha/beta phase junction) for self-powered solar-blind photodetectors. The small lattice mismatch and similar band gap between alpha- and beta-Ga2O3 will solve the two problems outlined above. The formation of alpha- and beta-Ga(2)O(3)is expected to result in a type-II band alignment, promoting separation of photogenerated carriers, which transfer through the junction to the corresponding electrodes. Herein, the alpha/beta phase junction of Ga2O3 vertically aligned nanorod arrays with a thickness-controllable beta-Ga2O3 shell layer are fabricated by a low-cost and simple process of hydrothermal and postannealing treatment. Two different types of self-powered alpha/beta-Ga2O3 phase junction-based photodetectors, in the form of solid-state type and photoelectrochemical type, are constructed and realized. Our analysis shows that the constructed photodetectors are capable of highly efficient detection of solar-blind signal without any bias voltage. This work demonstrates the usefulness of using the alpha/beta-Ga2O3 phase junction in a self-powered solar-blind photodetector, which is not only energy efficient, but also potentially workable in outer space, at the south and north pole, and other harsh environments without external power for a long time.
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