Journal
SURFACE ENGINEERING
Volume 36, Issue 6, Pages 660-664Publisher
TAYLOR & FRANCIS LTD
DOI: 10.1080/02670844.2020.1727687
Keywords
Brass; surfaces; nanostructures; superhydrophobicity; corrosion; electrochemical impedance spectroscopy; diffusion; impedance
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In this study, superhydrophobic surfaces were fabricated using 1H,1H,2H,2H-perfluorooctyltriethoxysilane monolayer deposition on thermally oxidized brass. The superhydrophobic surface showed a contact angle (CA) of 155 degrees with a CA hysteresis of 3.5 degrees. The corrosion behaviour of developed superhydrophobic surface was evaluated using potentiodynamic polarization and electrochemical impedance spectroscopy (EIS) studies in 3.5% NaCl solution. The superhydrophobic surface showed exceptional corrosion behaviour with nearly 21 times higher corrosion resistance compared to as-received (AS) brass. The EIS analysis suggests the presence of Warburg impedance in the AS brass indicating diffusion phenomena, while superhydrophobic brass surface showed a reversed loop in the low-frequency spectra, signifying significantly delayed kinetics of the electrochemical system. The study provides a facile, promising means of developing highly corrosion-resistant surfaces in engineering materials.
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