Journal
PROGRESS IN REACTION KINETICS AND MECHANISM
Volume 45, Issue -, Pages -Publisher
SAGE PUBLICATIONS LTD
DOI: 10.1177/1468678319825732
Keywords
Diformyltricyclodecanes; hydrogenation; Ru-Ni bimetallic catalyst; magnetic catalyst
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Funding
- Chinese Government ``Thousand Talent'' Program [Y42H291501]
- National Natural Science Foundation of China [U1139302]
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A series of magnetically separable catalysts based on Ru-Ni bimetallic compounds supported on Fe3O4 nanoparticles was prepared by the co-precipitation method. These catalysts were evaluated for diformyltricyclodecanes hydrogenation reactions, achieving 97% tricyclodecanedimethylol selectivity at 98% diformyltricyclodecanes conversion under mild conditions. The catalyst could be easily recovered by using the magnetic property of the iron oxide support. The catalysts were characterized with X-ray photoelectron spectroscopy, X-ray diffraction, and temperature-programmed reduction. These complementary characterization results suggested that the superior catalytic activity may be derived from the delicate synergy between Ru and Ni species.
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