Journal
ORGANIC LETTERS
Volume 22, Issue 5, Pages 1894-1898Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c00235
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Funding
- Excellence Initiative of Aix-Marseille University A*MIDEX
- French Investissement d'Avenir program
- CNRS
- MRES
- AMU
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A convenient and versatile procedure for the straightforward synthesis of substituted fluorenones as valuable scaffolds is described under rhodium catalysis. The present [2 + 2 + 2] cycloaddition reaction of diynes with 3-acetoxy or-3-alkoxyindenones as surrogates of the highly reactive benzocyclopentynone 2 pi partner allows the preparation of various fluorenone-type derivatives in good yields and provides an additional and tunable process for the generation of more challenging molecules with application in pharmaceutical, polymer, and material sciences.
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