4.6 Article

Role of matrix elements in the time-resolved photoemission signal

Journal

NEW JOURNAL OF PHYSICS
Volume 22, Issue 2, Pages -

Publisher

IOP PUBLISHING LTD
DOI: 10.1088/1367-2630/ab6eb1

Keywords

time- and angle-resolved photoemission spectroscopy (TR-ARPES); matrix-elements; topological insulators; ultrafast electron dynamics

Funding

  1. Max Planck-UBC-UTokyo Centre for Quantum Materials
  2. Canada First Research Excellence Fund, Quantum Materials and Future Technologies Program
  3. Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4779]
  4. Killam Steacie Memorial Fellowship
  5. Alfred P Sloan Steacie Memorial Fellowship
  6. Natural Sciences and Engineering Research Council of Canada's (NSERC's) Steacie Memorial Fellowship
  7. Alexander von Humboldt Fellowship
  8. Canada Research Chairs Program
  9. NSERC
  10. Canada Foundation for Innovation (CFI)
  11. British Columbia Knowledge Development Fund (BCKDF)
  12. CIFAR Quantum Materials Program
  13. Swiss National Science Foundation (SNSF) [P300P2_164649]
  14. MIUR through the PRIN 2015 Programme [2015C5SEJJ001]
  15. Universita Cattolica del Sacro Cuore [D.1, D.2.2, D.3.1]
  16. European Union's Horizon 2020 research and innovation programme [785219 GrapheneCore2]
  17. LANL Directors Postdoctoral Funding LDRD program XWVM
  18. US Department of Energy Office of Science, BESMSE Science of 100 Tesla programs
  19. Swiss National Science Foundation (SNF) [P300P2_164649] Funding Source: Swiss National Science Foundation (SNF)

Ask authors/readers for more resources

Time- and angle-resolved photoemission spectroscopy (TR-ARPES) provides access to the ultrafast evolution of electrons and many-body interactions in solid-state systems. However, the momentum- and energy-resolved transient photoemission intensity may not be unambiguously described by the intrinsic relaxation dynamics of photoexcited electrons alone. The interpretation of the time-dependent photoemission signal can be affected by the transient evolution of the electronic distribution, and both the one-electron removal spectral function as well as the photoemission matrix elements. Here we investigate the topological insulator Bi1.1Sb0.9Te2S to demonstrate, by means of a detailed probe-polarization dependent study, the transient contribution of matrix elements to TR-ARPES.

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