Journal
JOURNAL OF ELECTRONIC MATERIALS
Volume 49, Issue 3, Pages 2050-2057Publisher
SPRINGER
DOI: 10.1007/s11664-019-07883-3
Keywords
Lithium-sulfur batteries; electrochemical properties; decoration; MWCNTs; Co-PC interlayer
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Funding
- Jiangxi Scientific Fund [20142BBE50071]
- Jiangxi Education Fund [KJLD13006]
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In this paper, we develop a simple annealing method to prepare three-dimensional (3D) honeycomb porous carbon (Co-PC) as an interlayer material. Co2+ was introduced by redox reaction to improve the initial coulombic efficiency and boost the specific capacity of the electrodes; CoS obtained during the S melt-diffusion process served as redox catalyst. The 3D interconnected porous structure of the Co-PC interlayer was found to effectively adsorb polysulfide to inhibit the shuttle effect. Remarkable cycling stability was obtained, and a high reversible capacity of 803 mAh/g with a negligible fading rate of 0.024% per cycle at 1C was obtained after 200 cycles.
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