Article
Biophysics
Bing Li, Yunxiao Li, Chenchen Li, Jinghui Yang, Deling Liu, Huabin Wang, Rui Xu, Yong Zhang, Qin Wei
Summary: In this study, a novel split-type electrochemical immunosensor based on controlled release strategy was proposed for sensitive analysis and detection of tumor marker carbohydrate antigen 199 (CA19-9). The immunosensor showed wide linear concentration range and highly sensitive detection of CA19-9. It provides an innovative approach for trace detection of other biomarkers.
BIOSENSORS & BIOELECTRONICS
(2023)
Article
Chemistry, Analytical
Xue Wang, Dongquan Leng, Faying Li, Lei Liu, Xiang Ren, Jin Yong Lee, Huangxian Ju, Qin Wei
Summary: An efficient photoelectrochemical (PEC) split-type sensor based on a controlled release strategy was successfully established for ultrasensitive and accurate physiological monitoring, with improved visible light absorption efficiency and stability. The sensor separated the immune reaction from the photoelectrochemical conversion process, eliminating interference. The use of Cu2O nanocubes as labels and acid etching improved the sensitivity of the sensor. Under optimized conditions, the PEC sensor showed a wide concentration linear range and a low detection limit for CYFRA21-1 target detection.
ANALYTICA CHIMICA ACTA
(2023)
Article
Chemistry, Analytical
Xue Dong, Hanyu Wang, Xiang Ren, Hongmin Ma, Dawei Fan, Dan Wu, Qin Wei, Huangxian Ju
Summary: In this study, a mesoporous silica nanospheres (MSNs)-assisted split-type photoelectrochemical (PEC) aptasensor with in situ generation of Bi2S3 was proposed for reliable detection of prostate-specific antigen (PSA). The release of Na2S, induced by the reaction between PSA and aptamer, led to the formation of BiOI/BiOBr/Bi2S3 composite, altering the electron-hole transfer pathway and decreasing the photocurrent response. The sensor exhibited a linear range of 10 pg·mL-1-1 μg·mL-1 and a detection limit of 1.23 pg·mL-1, demonstrating satisfactory stability and anti-interference.
ANALYTICA CHIMICA ACTA
(2023)
Article
Chemistry, Analytical
Yu Bai, Dongquan Leng, Tao Feng, Xuan Kuang, Dawei Fan, Xiang Ren, Yuyang Li, Qin Wei, Huangxian Ju
Summary: A split-type photoelectrochemical immunosensor was designed to detect neuron-specific enolase (NSE), a tumor marker for small cell lung cancer found in nerve and neuroendocrine tissues. In this study, a heterogeneous In2O3/BiVO4 structure was developed using simplified successive ionic layer adsorption and reaction (s-SILAR). Immune recognition occurred in a 96-well plate, avoiding interference with biomolecule recognition. By regulating the degradation of the ZIF-8 protective layer, the split-type PEC immunosensor achieved sensitive detection of NSE.
SENSORS AND ACTUATORS B-CHEMICAL
(2023)
Article
Chemistry, Analytical
Luyao Liu, Chenglong Sun, Jialin Liu, Yun Du, Qingji Xie
Summary: This study investigated the photoelectrochemistry sandwich immunosensing of the lung cancer marker CYFRA21-1 using an In2O3/WO3 heterojunction modified fluorine-doped tin oxide (FTO) electrode as the photoanode and CdS quantum dots-polydopamine nanospheres as the secondary antibody label. Under optimized conditions, the photocurrent showed a linear relationship with the logarithm of CYFRA21-1 concentration, with a high sensitivity for CYFRA21-1 measurement.
Article
Chemistry, Analytical
Sethupathi Velmurugan, Thomas C-K Yang, Jyy-Ning Chen, Liu Zhi-Xiang
Summary: The synthesis of eco-friendly metal oxide pn junction composite with high visible light absorption and its photoelectrochemical monitoring on antibiotics were reported. The In2O3-CuO pn heterojunction composite exhibited high conductivity and stability for the detection of ornidazole, with a detection limit of 0.0092 nM. The sensor device showed practical applicability in various samples with recoveries above 95%, validated against electrochemical methods.
Article
Chemistry, Analytical
Dongqing Liu, Xinyu Bai, Jing Sun, Danyang Zhao, Chenghui Hong, Nengqin Jia
Summary: In this study, a novel molecularly imprinted photoelectrochemical (PEC) sensor based on hollow In2O3/In2S3 material was developed for sensitive detection of glutathione (GSH). The sensor exhibited excellent selectivity, a wide detection range, and a low detection limit, as well as excellent stability and selectivity.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Engineering, Electrical & Electronic
Cecilia I. Vazquez, Felipe Montero Bruni, Ana Maria Baruzzi, Rodrigo A. Iglesias
Summary: A non-enzymatic photoelectrochemical method using a CdS|TiO2 nanotubes photoanode is proposed for the detection of aqueous sulfide and ascorbic acid. The sensitivity of both the CdS|TiO2 and CdS|Pt photoanodes is high in the visible range, allowing for detection at micromolar levels for sulfide and ascorbic acid. However, the detection of H2O2 leads to the degradation of CdS and the release of Cd2+ ions into the analyte solution.
IEEE SENSORS JOURNAL
(2023)
Article
Chemistry, Analytical
Pei Miao, Mengjiao Hao, Chengfang Li, Wenshou Wang, Shenguang Ge, Xiaofeng Yang, Bing Geng, Biyan Ding, Jing Zhang, Mei Yan
Summary: A split-type photoelectrochemical (PEC) sensor based on Ti3C2/MgIn2S4 has been proposed for sensitive and accurate detection of miRNA-21. The Ti3C2/MgIn2S4 heterojunction effectively separates photogenerated electrons and holes, while a multifunctional PCN-224 nanocontainer amplifies the signal. The sensor achieved enhanced photocurrent response by releasing trapped glucose and utilizing glucose oxidase to generate hydrogen peroxide.
ANALYTICA CHIMICA ACTA
(2022)
Article
Chemistry, Multidisciplinary
Guo-Na Huo, Sha-Sha Zhang, Yue-Liu Li, Jia-Xing Li, Zhao Yue, Wei-Ping Huang, Shou-Min Zhang, Bao-Lin Zhu
Summary: Heterojunction structures formed by TiO2 nanotubes can enhance the photoelectric properties by preventing the recombination of electron-hole pairs. A CdS-TiO2NTs photoelectrochemical sensor was fabricated using the hydrothermal-impregnation method, showing good PEC performance under visible light.
Article
Chemistry, Analytical
Ben-Fang Xu, Qianan Li, Ping Qu, Xiao-Ru Xin, Ai-Jun Wang, Li-Ping Mei, Pei Song, Jiu-Ju Feng
Summary: A split-type photoelectrochemical (PEC) sensor was designed using magnetic-assisted exciton-plasmon interactions (EPI) to detect profenofos (PFF). Core-shell Bi2S3 nanorods@MoS2 nanosheets (Bi2S3 NRs@MoS2 NSs) heterostructure nanomaterial with excellent performance was synthesized and utilized as the photovoltaic conversion substrate and signal molecules absorption platform. The proposed PEC sensor demonstrated outstanding analytical performances, including a wide linear range, low detection limitation, excellent specificity, high stability, and applicability. Furthermore, it provided a new signal strategy for PEC biosensors and extended their application in environmental analysis.
Article
Chemistry, Physical
Hongfen Zhang, Fangmiao Liang, Baiyan Zhang, Sihan Li, Hongyuan Shang
Summary: The photoelectrochemical (PEC) performance of nano-semiconductor materials can be enhanced by preventing carrier recombination. Here, CdS/ xNiO nano-semiconductor materials were synthesized using atomic layer deposition (ALD) technique. The deposition of NiO effectively inhibited the carrier recombination rate of CdS. A glucose biosensor based on CdS/80NiO showed excellent PEC performance and was successfully developed for simple, fast, sensitive, and label-free glucose detection.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Physical
Ran Wu, Tao Liu, Xingtai Chen, Xi-Tao Yin
Summary: In this work, In2O3-modified Mn2O3 nanorod was prepared by a hydrothermal method, and the gas sensing performance of composites with different In/Mn ratios was investigated. The results showed that the composites exhibited high response, excellent selectivity, ultra-high resistance stability, and repeatability. This work provides a reference for designing multi-dimensional heterostructures and high-performance gas sensors.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Article
Materials Science, Ceramics
Sha-Sha Zhang, Jing Tian, Zhao Yue, Guo-Na Huo, Zhi-Xin Hu, Shou-Min Zhang, Wei-Ping Huang, Bao-Lin Zhu
Summary: Heterojunction technology can improve the efficiency of photoelectric conversion and be used to manufacture high-sensitivity, stable, and selective biosensors.
CERAMICS INTERNATIONAL
(2022)
Article
Multidisciplinary Sciences
Hefeng Zhang, Shengliang Qi, Haidong Wang, Guanghui Zhang, Kaixin Zhu, Weiguang Ma
Summary: In this study, g-C3N4@CdS composites were used as sensing elements in a photoelectrochemical platform for the rapid, selective, and sensitive detection of L-cysteine. The system exhibited a wide determination range (5-190 μM), a very low detection limit (1.56 μM), fast response time, and good long-term stability (approximately 1 month). The g-C3N4@CdS composites provided better optoelectronic function than bare CdS materials due to their high photon-to-current conversion efficiency and excellent anti-photocorrosion properties. Additionally, without any separation procedures, low concentrations of L-cysteine were successfully detected in human urine samples, consistent with the results of chemiluminescence.
Article
Nanoscience & Nanotechnology
Xianzhen Song, Xinrong Shao, Li Dai, Dawei Fan, Xiang Ren, Xiaojun Sun, Chuannan Luo, Qin Wei
ACS APPLIED MATERIALS & INTERFACES
(2020)
Article
Nanoscience & Nanotechnology
Cui Song, Xiaojian Li, Lihua Hu, Tengfei Shi, Dan Wu, Hongmin Ma, Yong Zhang, Dawei Fan, Qin Wei, Huangxian Ju
ACS APPLIED MATERIALS & INTERFACES
(2020)
Article
Chemistry, Analytical
Rui Xu, Jingshuai Li, Lei Liu, Xuejing Liu, Dawei Fan, Wei Cao, Hongmin Ma, Qin Wei
ANALYTICA CHIMICA ACTA
(2020)
Article
Chemistry, Analytical
Jinhui Feng, Faying Li, Yanrong Qian, Xu Sun, Dawei Fan, Huan Wang, Hongmin Ma, Qin Wei
SENSORS AND ACTUATORS B-CHEMICAL
(2020)
Article
Chemistry, Analytical
Chao Wang, Lei Liu, Xuejing Liu, Yu Chen, Xueying Wang, Dawei Fan, Xuan Kuang, Xu Sun, Qin Wei, Huangxian Ju
SENSORS AND ACTUATORS B-CHEMICAL
(2020)
Article
Nanoscience & Nanotechnology
Yanrong Qian, Jinhui Feng, Rui Xu, Dawei Fan, Yu Du, Xiang Ren, Qin Wei, Huangxian Ju
ACS APPLIED MATERIALS & INTERFACES
(2020)
Article
Geochemistry & Geophysics
Jingui Xu, Dawei Fan, Dongzhou Zhang, Maining Ma, Yi Zhou, Sergey N. Tkachev, Wenge Zhou, Przemyslaw K. Dera
Summary: This study investigated the phase transitions of natural and synthetic orthopyroxenes under high pressure and temperature conditions, and found possible metastable phases under certain pressure and temperature conditions. The composition was found to influence the pressures of the phase transitions. These findings provide valuable insights into the behavior of orthopyroxenes in subducting slabs.
JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH
(2022)
Article
Geochemistry & Geophysics
Jingui Xu, Dawei Fan, Bo Li, Sergey N. Tkachev, Vitali B. Prakapenka, Dongzhou Zhang, Guangzhong Yang, Yi Zhou, Wenge Zhou
Summary: Single-crystal X-ray diffraction and Brillouin spectroscopy experiments were conducted on a natural Cr-pyrope at high pressure and high temperature, revealing the elastic properties and density calculations can be accurately approximated using an end-member model in the subcontinental lithospheric mantle (SCLM).
GEOCHEMISTRY GEOPHYSICS GEOSYSTEMS
(2022)
Article
Geochemistry & Geophysics
Zhilin Ye, Jingui Xu, Dawei Fan, Dongzhou Zhang, Wenge Zhou, Hongsen Xie
Summary: This study reveals the pressure-induced, irreversible amorphous transformation of tephroite, providing insights into its behavior under high-pressure conditions and suggesting its significance in the mantle transition zone.
AMERICAN MINERALOGIST
(2023)
Article
Chemistry, Analytical
Jiajun Liu, Yu Du, Aiping Guo, Nuo Zhang, Lei Liu, Dawei Fan, Xue Dong, Qin Wei, Huangxian Ju
Summary: In this study, a sandwich sensing platform was developed using silica-coated silver nanoparticles as a luminescent material and cerium dioxide as a signal quencher for sensitive neuro-specific enolase detection. The core-shell structure protected the silver nanoparticles and improved their luminescence properties. Amino-functionalized cerium dioxide efficiently diminished the luminescence signal, resulting in a highly sensitive and accurate detection mode. This detection strategy showed a powerful capability for biomolecule detection.
Article
Chemistry, Multidisciplinary
Rui Xu, Yu Du, Dongquan Leng, Lei Liu, Yuyang Li, Xiang Ren, Dawei Fan, Huan Wang, Qin Wei
CHEMICAL COMMUNICATIONS
(2020)
Article
Chemistry, Analytical
Yu Du, Xiaojian Li, Xiang Ren, Huan Wang, Dan Wu, Hongmin Ma, Dawei Fan, Qin Wei
Article
Chemistry, Multidisciplinary
Xin Liu, Chunzhu Bao, Xinrong Shao, Yong Zhang, Nuo Zhang, Xu Sun, Dawei Fan, Qin Wei, Huangxian Ju
NEW JOURNAL OF CHEMISTRY
(2020)
Article
Chemistry, Multidisciplinary
Yuewen Li, Rui Xu, Dong Wei, Rui Feng, Dawei Fan, Nuo Zhang, Qin Wei
NEW JOURNAL OF CHEMISTRY
(2020)