Journal
ORGANIC ELECTRONICS
Volume 77, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.orgel.2019.105546
Keywords
Perovskite light-emitting devices; Mixed-cation perovskites; Large-group ammonium bromide; Defect passivation
Funding
- National Natural Science Foundation of China [11474232,11374242, 61874016]
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In this work, we report the morphology, crystal structure, photo-physics, and electroluminescence characteristics of perovskite materials containing a mixture of methylammonium (MA) and ethylammonium (EA) cations with the form MA(x)EA((1-x))PbBr(3). Hybridization of MA and EA cations simultaneously increases the photoluminescence quantum yield and thermal-, environmental-, and photo-stability of perovskite materials as the result of crystal structure modification, defect passivation, and morphology improvement. The addition of a large-group ammonium bromide further reduces defect density and raises the maximum external quantum efficiency of related light-emitting devices to 14.5%. These findings enrich the library of A-site cations for efficient perovskite light-emitting devices and may pave the way toward the realization of high performance multication perovskites-based light-emitting devices.
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