Journal
JOURNAL OF MATERIALS SCIENCE
Volume 55, Issue 7, Pages 2937-2946Publisher
SPRINGER
DOI: 10.1007/s10853-019-04145-9
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Funding
- Key Scientific Research Project of Suzhou University [2019yzd02]
- Provincial Natural Science Foundation of Anhui [1908085ME120]
- Research platform Project of Suzhou University [2016ykf05]
- Primary Research and Development Program of Anhui Province [201904a05020087]
- Outstanding Youth Talents in Anhui Provincial Education Department
- Foundation of Suzhou University [2016XJXS05, 2018SZXYDZXZ02]
- Innovative Research Team of Anhui Provincial Education Department [2016SCXPTTD]
- Key Discipline of Material Science and Engineering of Suzhou University [2017XJZDXK3]
- [2017GXBJZD47]
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High-quality perovskite films are the key factor in manufacturing high-performance devices. In this work, we for the first time use carbon quantum dots (CQDs) as additive in the methylammonium iodide solution for high-quality CH3NH3PbI3 (MAPbI(3)) films. Appropriate concentration of CQDs (0.04 mg ml(-1)) can passivate the crystal defects, improve the crystallinity, increase the grain size and reduce the grain boundary of MAPbI(3) film. Various characterization results show that CQDs additive can reduce trap-state density, decrease carrier recombination and improve photoelectric performance. Compared with the pristine device, the average power conversion efficiency (PCE) of CQD-modified MAPbI(3) device was increased from 15.8 +/- 0.37% to 18.81 +/- 0.45%, and the maximum PCE of champion device was increased from 16.21 to 19.17%. In this study, we propose a simple method for the preparation of stable and efficient inverted planar structure perovskite solar cells using CQD additives in a two-step spin-coated deposition method.
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