Journal
ENVIRONMENTAL SCIENCE & TECHNOLOGY
Volume 53, Issue 21, Pages 12594-12601Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.est.9b04488
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Funding
- Department of Energy, Office of Fossil Energy
- NASA Atmospheric Composition Modeling and Analysis Program (ACMAP)
- U.S. Environmental Protection Agency [RD835871]
- [DE-AC02-06CH11357]
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The TROPOspheric Monitoring Instrument (TROPOMI) is used to derive top-down NOx emissions for two large power plants and three megacities in North America. We first re-process the vertical column NO2 with an improved air mass factor to correct for a known systematic low bias in the operational retrieval near urban centers. For the two power plants, top-down NOx emissions agree to within 10% of the emissions reported by the power plants. We then derive top-down NOx emissions rates for New York City, Chicago, and Toronto, and compare them to projected bottom-up emissions inventories. In this analysis of 2018 NOx emissions, we find a +22% overestimate for New York City, a -21% underestimate in Toronto, and good agreement in Chicago in the projected bottom-up inventories when compared to the top-down emissions. Top-down NOx emissions also capture intraseasonal variability, such as the weekday versus weekend effect (emissions are +45% larger on weekdays versus weekends in Chicago). Finally, we demonstrate the enhanced capabilities of TROPOMI, which allow us to derive a NOx emissions rate for Chicago using a single overpass on July 7, 2018. The large signal-to-noise ratio of TROPOMI is well-suited for estimating NOx emissions from relatively small sources and for sub-seasonal timeframes.
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