Journal
CHEMICAL ENGINEERING JOURNAL
Volume 375, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2019.122054
Keywords
Supercapacitors; Dual redox-active ions electrolyte; BiBr3
Categories
Funding
- National key research and development program [2016YFB0901600]
- Science and Technology Commission of Shanghai [16JC1401700]
- National Science Foundation of China [21871008, 51672301]
- Key Research Program of Chinese Academy of Sciences [QYZDJ-SSW-JSC013, KGZD-EW-T06]
- CAS Center for Excellence in Superconducting Electronics
- Youth Innovation Promotion Association CAS
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Capacitor-like and battery-like energy storage characteristics can be incorporated into a single cell to achieve optimal performance metrics through adding dual redox-active ions Bi3+/Br- to electrolyte. By adding dual redox-active ions to traditional electrolyte of carbon-based supercapacitor, redox reactions occur at each electrolyte/electrode interface simultaneously to store energy, exhibiting significant charge and discharge platforms which are battery-like energy storage characteristics. Moreover, a specific capacitance of 1150 F/g and an energy density of 61.8 Wh/kg are achieved at 2 A/g, surpassing most of the state-of-the-art work.
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