Journal
JOURNAL OF SOLID STATE CHEMISTRY
Volume 276, Issue -, Pages 302-308Publisher
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jssc.2019.05.027
Keywords
Low temperature; Electron transport layer; C-60; Perovskite solar cells; Ionic-liquid; Interfacial modification
Funding
- National Natural Science Foundation of China [51772095]
- Fundamental Research Funds for the Central Universities [2018MS040, 2018ZD07, JB2018135]
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Low temperature solution-processed C-60 exhibits favorable electron mobility and band alignment, thus it is widely used to modify the interfaces between perovskite film and electron transport layer (ETL) in n-i-p planar heterojunction perovskite solar cells (PSCs). However, when C-60 was used as an independent ETL, PSCs exhibit poor performance. Herein, We have modified solution-processed C-60-based ETL with a solid-state ionic-liquid (1-ethyl-3-methylimidazolium iodide ([EMIM]I)). Using this interfacial modification method, we fabricated n-i-p planar heterojunction PSCs with optimized power conversion efficiency (PCE) of 15.09%, which was superior to that of PSCs based on unmodified C-60 ETL layer (12.11%). This work describes a novel method for low-temperature processing of efficient n-i-p PSCs.
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