Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 25, Issue 67, Pages 15228-15232Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201903829
Keywords
coordination chemistry; heterometallic complexes; lanthanides; ligand design; quantum computing
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Funding
- Spanish MINECO [CTQ2015-68370-P, PGC2018-098630-B-I00, MAT2017-86826-R, RTI2018-096075-B-C21]
- Juan de la Cierva program [IJCI-2016-29901]
- Aragon government (DGA) [E09_ 17R Q-MAD, PLATON E31_17R]
- QUANTERA [PCI2018-093106, PCI2018-093116]
- DOE Office of Science User Facility [DE-AC02-05CH11231]
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The combination of two different beta-diketone ligands facilitates the size-controlled assembly of pure heterometallic [LnLn ' Ln] linear compounds thanks to two different coordination sites present in the molecular scaffold. [HoCeHo], [ErCeEr], and [YbCeYb] analogues are presented here and are characterized both in the solid state and in solution, demonstrating the selectivity of this unique method to produce heterometallic 4f molecular entities.
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