Article
Biochemistry & Molecular Biology
Yunqing Zhu, Bingqing Li, Yongming Wang, Tian Wang
Summary: Electrocatalytic oxidation (ECO) is a highly efficient and environmentally friendly method for water treatment. This study focuses on the preparation of high-performance anodes with long service lifetimes. Porous Ti/RuO2-IrO2@Pt, Ti/RuO2-TiO2@Pt, and Ti/Y2O3-RuO2-TiO2@Pt anodes were fabricated using modified micro-emulsion and vacuum impregnation methods. These anodes exhibited large electrochemically active areas and long service lives. The Ti/Y2O3-RuO2-TiO2@Pt anode showed the highest degradation efficiency for tetracycline and consumed the lowest energy.
Article
Environmental Sciences
Xu Zhu, Weiwu Hu, Chuanping Feng, Nan Chen, Hongyan Chen, Peijing Kuang, Yang Deng, Linlin Ma
Summary: The electrocatalytic properties of Ti/RuO2-SnO2 and Ti/RuO2-IrO2 anodes in different electrolytes were studied for aniline degradation. Ti/RuO2-SnO2 showed higher activity in Na2SO4 electrolyte, while Ti/RuO2-IrO2 was more effective in NaCl electrolyte. The presence of Fe2+ can decrease TOC removal efficiency, especially for Ti/RuO2-SnO2.
Article
Environmental Sciences
Yunxia Niu, Yue Yin, Runyu Xu, Zhinian Yang, Jia Wang, Duo Xu, Yue Yuan, Jinlong Han, Hao Wang
Summary: In this study, a stable Ti/SnO2-RuO2 anode was prepared successfully and used for the degradation of low concentration CFX using green and sustainable electrocatalytic oxidation technology. The effects of various parameters on the degradation efficiency were discussed, and the optimal conditions for CFX removal were identified. The electrochemical analysis and Fourier transform infrared spectroscopy provided insights into the degradation efficiency and process.
Article
Environmental Sciences
Xianni Song, Xu Chen, Shuchi Zhang, Donglei Wu
Summary: The electrolytic process conditions for the electrochemical oxidation (EO) of composting leachate biochemical effluent (CLBE) were optimized using the response surface methodology (RSM). Comparative studies were conducted to investigate the failure characteristics of Ti/RuO2-IrO2 anodes in different electrolyte solutions. The optimization results showed a high removal rate for COD, NH3-N, and TN, and the failure mechanism of the Ti/RuO2-IrO2 anodes was clarified through electrochemical and material characterizations.
Article
Green & Sustainable Science & Technology
Guozhen Zhang, Xingxing Huang, Jinye Ma, Fuping Wu, Tianhong Zhou
Summary: The study developed two-dimensionally stable anodes to successfully degrade organic pollutants from pharmaceutical wastewater through electrochemical oxidation, and discussed and optimized the electrocatalytic oxidation conditions under different parameters.
Article
Electrochemistry
Shuna Liu, Ben Yang, Anran Zuo, Yongming Tang
Summary: Ti/SnO2-Sb/Fe-PVP-PbO2 anodes were prepared and their electrocatalytic properties were investigated. The inclusion of Fe improved the stability of the anodes, while PVP enhanced their electrocatalytic activity. The co-doped anodes showed even higher stability and electrocatalytic activity, and the degradation pathway of MO was proposed.
JOURNAL OF THE ELECTROCHEMICAL SOCIETY
(2023)
Article
Chemistry, Multidisciplinary
Xuyang Hu, Hao Dong, Yinghao Zhang, Baihui Fang, Wenqiang Jiang
Summary: In this study, electrochemical oxidation was employed to degrade DMF, with the optimal operational conditions identified and four degradation pathways proposed. The DMF degradation was more thorough under optimal conditions.
Article
Electrochemistry
Naichuan Yu, Hanfei Cao, Xintong Hong, Xianhe Mao, Tongzhen Li, Hao Yuan, Jingnan Li, Fuchen Luo, Mingyu Li
Summary: This study compares the performance difference between PbO2 electrode and RuO2-IrO2 electrode, and finds that the former is suitable for the degradation of phenol, while the latter is suitable for the degradation of crystal violet.
JOURNAL OF SOLID STATE ELECTROCHEMISTRY
(2023)
Article
Engineering, Chemical
Wenlan Ji, Weiwei Li, Tian C. Zhang, Yuan Wang, Shaojun Yuan
Summary: To reduce the global hazards of arsenic, arsenic-containing water needs to be purified. This study synthesized dimensionally stable TNTAs/SnO2/RuO2 anodes for efficient electrocatalytic oxidation of As(III) by successively electrodepositing SnO2 and RuO2 nanoparticles on TiO2 nanotube arrays. The optimized TNTAs/SnO2/RuO2-10 anode exhibited excellent electrochemical stability and longer service lifetime, with an oxidation conversion efficiency of As(III) still maintained at 98% even after 11 cycles of usage.
SEPARATION AND PURIFICATION TECHNOLOGY
(2023)
Article
Chemistry, Applied
Weida Wang, Ke Wang, Wenting Hao, Tingting Zhang, Yijie Liu, Linghong Yu, Weiping Li
Summary: In this study, Ti/SnO2-RuO2 electrodes with different Yb contents were prepared and their surface morphology, crystal structure, and electrochemical properties were characterized. The results showed that 1.5% Yb doping increased the oxygen precipitation potential and electrocatalytic oxidation activity of the electrode. Under certain conditions, the electrode doped with 1.5% Yb effectively removed COD, TOC, and UV254 from coking wastewater.
JOURNAL OF RARE EARTHS
(2022)
Article
Environmental Sciences
Guangfei Gao, Yinghao Zhang, Chuanxing Zhang, Yanfeng Li, Fengchun Li, Yuhai He, Luwei Zhai, Ling Li, Xia Chen
Summary: This study investigated the degradation of residual levofloxacin (LEV) in the environment using the electrochemical anodic oxidation method. The Ti/RuO2-TiO2-SnO2 electrode demonstrated the highest degradation efficiency for LEV among the three different anodes tested. Factors such as electrode spacing, current strength, electrolyte concentration, and pH were found to affect the degradation of LEV. The optimal conditions for LEV degradation using the Ti/RuO2-TiO2-SnO2 electrode were determined. The study also revealed the mechanism and intermediate products of LEV degradation.
WATER AIR AND SOIL POLLUTION
(2023)
Article
Engineering, Environmental
Chao Yang, Lin Lin, Shanshan Shang, Shengshou Ma, Feiyun Sun, Kaimin Shih, Xiao-yan Li
Summary: This study introduces an innovative electrochemical wastewater treatment technology using packed bead-electrodes as a dynamic electrocatalytic filter, which expands the electroactive volume and greatly enhances the efficiency of electrochemical degradation of micropollutants. This technology has the potential to revolutionize electrochemical wastewater treatment and effectively control emerging pollutants in the water environment.
Article
Engineering, Environmental
Abhinesh Kumar Prajapati
Summary: The study examined the application of sono-electrocoagulation process in treating industrial wastewater, with the Fe-Fe electrode combination showing the best efficiency in COD and color removal. The operating cost of the process was found to be $1.39/m3.
PROCESS SAFETY AND ENVIRONMENTAL PROTECTION
(2021)
Article
Chemistry, Multidisciplinary
Chuan Wang, Zhifen Cao, Hongtao Huang, Hong Liu, Sha Wang
Summary: In this study, Co3O4/Ti electrodes were prepared by electrodeposition for the electrocatalytic reduction of nitrate. The results showed that Co3O4/Ti can effectively remove nitrate with low energy consumption and high current efficiency.
FRONTIERS IN CHEMISTRY
(2022)
Article
Engineering, Environmental
Shuaishuai Man, Dehui Luo, Qing Sun, Haifeng Yang, Hebin Bao, Ke Xu, Xuzhong Zeng, Miao He, Zehao Yin, Li Wang, Zhihong Mo, Wenjing Yang, Xueming Li
Summary: In this study, a highly conductive MXene (Ti3C2Tx) was fabricated for the first time using electrophoretic deposition (EPD) as an interlayer to prepare a novel PbO2 electrode. The Ti3C2Tx interlayer significantly improved the electrochemical performance of the EPD-2.0/PbO2 electrode, reducing the charge transfer resistance, increasing the number of active sites, and enhancing the generation ability of ·OH radicals. Experimental results showed that the EPD-2.0/PbO2 electrode exhibited promising potential for the electrochemical degradation of basic fuchsin (BF).
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Jian Zhang, Hongyan Yuan, Yanping Huang, Shuting Kan, Yufeng Wu, Manman Bu, Yang Liu, Ping He, Hongtao Liu
Summary: A novel sodium-rich tunnel-type Na0.6MnO2 material was reported in this study, fancily prepared with the guidance of CTAB surfactant, exhibiting outstanding cycling durability and high discharge capacity. The sodium-rich tunnel-structured manganese oxide provides a new perspective for engineering high-performance SIB cathode materials.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Environmental Sciences
Shouxian Chen, Ping He, Xuejiao Wang, Feng Xiao, Pengcheng Zhou, Qihang He, Lingpu Jia, Faqin Dong, Hui Zhang, Bin Jia, Hongtao Liu, Bin Tang
Summary: The Ti/PbO2 Co-Sm electrode exhibited the highest electrocatalytic activity for atrazine degradation compared to other electrodes, achieving a maximum degradation efficiency of 92.6% and COD removal efficiency of 84.5% under optimized conditions. The degradation mechanism of atrazine was proposed based on the detection of degradation intermediates, suggesting Ti/PbO2 Co-Sm as a promising electrode for atrazine degradation.
Article
Environmental Sciences
Shouxian Chen, Ping He, Pengcheng Zhou, Xuejiao Wang, Feng Xiao, Qihang He, Jing Li, Lingpu Jia, Hui Zhang, Bin Jia, Bin Tang
Summary: A novel GCN/CNT doped Ti/PbO2 anode was constructed for effective degradation of ACE wastewater, achieving removal efficiencies of 83.2% for ACE and 76.3% for chemical oxygen demand under optimal conditions. The excellent electrocatalytic activity of the Ti/PbO2-GCN-CNTanode for ACE oxidation is attributed to the effective suppression of oxygen evolution and enhanced electron transfer.
Article
Chemistry, Physical
Xuejiao Wang, Qihang He, Qianao Ge, Tongxing Fu, Shouxian Chen, Pengcheng Zhou, Feng Xiao, Ping He, Lingpu Jia, Bin Jia, Hui Zhang, Kai Pan, Hongtao Liu
Summary: Bacterial cellulose based carbon nanofiber (BCCNF) has been highlighted for its 3D network structure, and a series of nanocotton-like Co-B-P/BCCNF electrocatalysts have been designed and prepared, exhibiting excellent catalytic performances for water splitting with low overpotentials. This indicates great potential for large-scale hydrogen production.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Materials Science, Multidisciplinary
Xuejiao Wang, Shouxian Chen, Pengcheng Zhou, Feng Xiao, Qihang He, Ping He, Lingpu Jia, Bin Jia, Hui Zhang, Hongtao Liu, Kai Pan, Ying Xie
Summary: Nanocoral-like bimetallic Co-Mo carbide/nitrogen-doped carbon electrocatalysts exhibit superior electrocatalytic activity and stability for hydrogen evolution reaction, which can serve as promising candidates to substitute noble metal catalysts for green and renewable hydrogen production through electrocatalytic water splitting.
JOURNAL OF MATERIALS SCIENCE
(2021)
Article
Materials Science, Multidisciplinary
Qihang He, Xuejiao Wang, Pengcheng Zhou, Qianao Ge, Tongxing Fu, Shouxian Chen, Feng Xiao, Peilin Yang, Ping He, Lingpu Jia, Dingming Yang
Summary: Nanocoral-like cerium-activated cobalt selenide (Ce-CoSe2) nanocomposites were successfully prepared to enhance the oxygen evolution reaction (OER) catalytic activity. The Ce-CoSe2 catalyst exhibited remarkable OER performance with low overpotential and long-term stability, providing a simple and feasible pathway for designing metal dichalcogenides for green and renewable hydrogen production.
JOURNAL OF MATERIALS SCIENCE
(2021)
Article
Microbiology
Xiujuan Gu, Qi Cheng, Ping He, Yan Zhang, Zhengfang Jiang, Yali Zeng
Summary: The new nanomedicine antibacterial agent DHA-CS NPs shows excellent antibacterial effect on drug-resistant TB strains by disrupting the cell wall, indicating potential for TB treatment.
FRONTIERS IN MICROBIOLOGY
(2021)
Article
Materials Science, Multidisciplinary
Shuai (Marshall) Yang, Jinbao Huang, Jian Chen, James Joseph Noel, Ivan Barker, Jeffrey Daniel Henderson, Ping He, Haiping Zhang, Hui Zhang, Jesse Zhu
Summary: Powder coatings with zinc phosphate additives were studied in this research. The anti-corrosive performance of the coatings was improved, as confirmed by neutral salt spray and electrochemical tests. The optimized additive dosage was determined to be 2% for most coating systems, with performance improvements of up to one order of magnitude. The study also identified a synergistic effect between the additive and filler.
Article
Chemistry, Physical
Feng Xiao, Pengcheng Zhou, Ruixue Weng, Peilin Yang, Weishan Tang, Lei Liao, Yuan Wang, Maojie Zhao, Wenxi Zhang, Ping He, Bin Jia
Summary: A self-supporting electrode with outstanding catalytic activity and long-term stability has been fabricated by decorating CeO2 on Co-Mn-S nanosheets. The electrode exhibits quick Faradic process and favorable OER kinetics, making it a highly efficient electrocatalyst for OER.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Multidisciplinary
Lingpu Jia, Juan Hao, Long Yang, Jun Wang, Lijuan Huang, Kunping Liu
Summary: A novel direct electrochemical sensor based on a PDPP/GO/GCE nanocomposite-modified electrode was developed for the detection of chloramphenicol (CAP). The introduction of PDPP effectively improved the electrocatalytic activity of the sensor, as confirmed by cyclic voltammetry. The PDPP/GO/GCE exhibited a significant response signal to CAP, with a wide linear range and low limit of detection. The sensor also demonstrated satisfactory anti-interference, reproducibility, and stability.
Article
Chemistry, Physical
Pengcheng Zhou, Feng Xiao, Ruixue Weng, Quanguo Huang, Lei Wang, Qihang He, Weishan Tang, Peilin Yang, Rong Su, Ping He, Bin Jia, Liang Bian
Summary: The introduction of a carbon scaffold has improved the energy storage performance of polyindole. In this study, nitrogen-doped porous carbon materials are integrated with polyindole through emulsion polymerization to form composites. The morphology and size of the composites can be controlled by adjusting the carbon content. The resulting electrode exhibits high specific capacitance and cycling stability in sulfuric acid electrolyte. Moreover, the assembled asymmetric supercapacitor shows high specific energy and excellent cycling stability.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Article
Engineering, Environmental
Feng Xiao, Yanxia Cheng, Pengcheng Zhou, Shouxian Chen, Xuejiao Wang, Ping He, Xiaoqin Nie, Faqin Dong
Summary: A novel luffa cylindrica adsorbent modified with carboxyl and amidoxime groups was successfully prepared and demonstrated effective U(VI) uptake. The adsorbent showed outstanding performance under optimal conditions and could be efficiently regenerated for repeated use.
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
(2021)