4.8 Article

3D strain-induced superconductivity in La2CuO4+δ using a simple vertically aligned nanocomposite approach

Journal

SCIENCE ADVANCES
Volume 5, Issue 4, Pages -

Publisher

AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/sciadv.aav5532

Keywords

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Funding

  1. Engineering and Physical Sciences Research Council [EP/N509620/1]
  2. China Scholarship Council
  3. Cambridge Commonwealth, European and International Trust
  4. St. John's College
  5. EPSRC [EP/P026311/1, EP/N017242/1]
  6. ISF F.I.R.S.T. program [687/16]
  7. U.S. Department of Energy's National Nuclear Security Administration [DE-NA0003525]
  8. U.S. NSF [DMR-1565822]
  9. University of Cambridge
  10. National Natural Science Foundation of China [21872116]
  11. Harry de Jur Chair in Applied Science
  12. EPSRC [EP/N017242/1] Funding Source: UKRI

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A long-term goal for superconductors is to increase the superconducting transition temperature, T-C. In cuprates, T-C depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simply grown, self-assembled, vertically aligned nanocomposite thin films of La2CuO4+delta + LaCuO3, by strongly increasing out-of-plane distances without reducing in-plane distances (three-dimensional strain engineering), we achieve superconductivity up to 50 K in the vertical interface regions, spaced similar to 50 nm apart. No additional process to supply excess oxygen, e.g., by ozone or high-pressure oxygen annealing, was required, as is normally the case for plain La2CuO4+delta. films. Our proof-of-concept work represents an entirely new approach to increasing T-C in cuprates or other superconductors.

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