4.6 Article

Equivalence of RABBITT and Streaking Delays in Attosecond-Time-Resolved Photoemission Spectroscopy at Solid Surfaces

Journal

APPLIED SCIENCES-BASEL
Volume 9, Issue 3, Pages -

Publisher

MDPI
DOI: 10.3390/app9030592

Keywords

attosecond; streaking; RABBITT; photoemission; time-resolved photoemission; photoemission delay; photoelectron; photoelectron spectroscopy; photoeffect; chronoscopy

Funding

  1. German Research Foundation within Priority Program SPP Quantum Dynamics in Tailored Intense Fields [PF317/10-1]

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The dynamics of the photoelectric effect in solid-state systems can be investigated via attosecond-time-resolved photoelectron spectroscopy. This article provides a comparison of delay information accessible by the two most important techniques, attosecond streaking spectroscopy and reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) at solid surfaces, respectively. The analysis is based on simulated time-resolved photoemission spectra obtained by solving the time-dependent Schrodinger equation in a single-active-electron approximation. We show a continuous transition from the few-cycle RABBITT regime to the streaking regime as two special cases of laser-assisted photoemission. The absolute delay times obtained by both methods agree with each other, within the uncertainty limits for kinetic energies >10 eV. Moreover, for kinetic energies >10 eV, both streaking delay time and RABBITT delay time coincide with the classical time of flight for an electron propagating from the emitter atom to the bulk-vacuum interface, with only small deviations of less than 4 as due to quantum mechanical interference effects.

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