Journal
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY
Volume 77, Issue -, Pages 280-290Publisher
ELSEVIER SCIENCE INC
DOI: 10.1016/j.jiec.2019.04.049
Keywords
Advanced oxidation processes; Nanocatalyst; Ultrasonic-assisted process; Metal-organic framework
Funding
- University of Tabriz and Gebze Technical University
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Herein, Fe3O4@MOF-2 (MOF: metal-organic framework) nanocomposite, as a heterogeneous nano catalyst, was applied to activate persulfate (PS) in the attendance of ultrasonic (US) irradiation (Fe3O4@MOF-2/US/PS) for degradation of diazinon. The evaluation results showed that, in the acidic solution (pH = 3), the reaction rate constant of Fe3O4@MOF-2/US/PS system (0.0546 min(-1)) was more than 6-folds than that of the US/PS system (0.0079 min(-1)). Reducing the diazinon concentration, along with raising the Fe(3)O(0)4@MOF-2 dosage and the US bath power favored the degradation of diazinon. It was found that Fe3O4@MOF-2 had fine catalytic performance and reuseibility. The diazinon decomposition pathway was proposed by GC-MS analysis. (C) 2019 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
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