Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 361, Issue 15, Pages 3543-3547Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201900380
Keywords
cycloaddition; 1; 6-enynes; oxabenzonorbornadiene; [Rh(COD)(2)]BF4; (R)-Xyl-P-Phos
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Funding
- National Natural Science Foundation of China [21302162, 21572198]
- Applied Basic Research Project of Yunnan Province [2017FA004, 2018FB021]
- Yunnan Provincial Key Laboratory Construction Plan Funding of Universities
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The asymmetric [2+2+2] cycloaddition reactions of 1,6-enynes and oxabenzonorbornadienes was accomplished by using the complex of [Rh(COD)(2)]BF4 and (R)-Xyl-P-Phos as chiral catalyst. A range of 1,6-enynes and oxabenzonorbornadienes were well tolerated in the cycloaddition reaction, which afforded various polycyclic products with asymmetric quaternary carbon centers generally in excellent enantioselectivities.
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