Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 55, Issue 48, Pages 15137-15141Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201608724
Keywords
cross-coupling; dearomatization; homogeneous catalysis; naphthol; palladium
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Funding
- National Basic Research Program of China from MOST [2015CB856600, 2016YFA0202900]
- National Natural Science Foundation of China [21332009, 21421091]
- Chinese Academy of Sciences
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The first Pd-0-catalyzed intermolecular arylative dearomatization of beta-naphthols with aryl halides is described. It was found that Q-Phos could facilitate the palladium-catalyzed cross-coupling-type dearomatization of b-naphthols, while avoiding O-arylation, to construct 2-naphthalenones in excellent yields and with high chemoselectivity.
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