Journal
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
Volume 7, Issue 4, Pages 3647-3670Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.8b05463
Keywords
Porous materials; Scale-up production; Green synthesis; Continuous processing
Categories
Funding
- National University of Singapore [CENGas R-261-508-001-646]
- Ministry of Education Singapore (MOE AcRF Tier 1) [R-279-000-472-112, R-279-000-540-114]
- Agency for Science, Technology and Research [PSF 1521200078, IRG A1783c0015, IAF-PP A1789a0024]
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Advanced porous materials (APMs) constructed from structure -encoded building blocks present an unprecedented degree for molecular design, and have demonstrated class-leading performance in numerous applications. However, the development of economically viable and sustainable synthetic means of production is a critical prerequisite to translate APMs to real-world applications. In this Perspective, we first consider the diverse synthetic routes to APMs-metal/covalent organic frameworks (MOFs/COFs), porous organic polymers (POPs) and porous molecular solids-and highlight the challenges for scalable and sustainable synthesis. Subsequently, we illustrate concepts to guide the sustainable synthesis of APMs with recent examples in the literature. Lastly, we present our outlook for the translation of molecular design to scalable APM production.
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