Journal
ORGANIC LETTERS
Volume 21, Issue 3, Pages 807-811Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b04084
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Funding
- Spanish Ministry of Economy and Competitiveness [CTQ2016-74878-P, CTQ2017-87840-P]
- IRB Barcelona
- European Regional Development Fund (AEI/FEDER, UE)
- Catalan Government [2017SGR1472]
- ICREA Foundation (ICREA Academia award)
- Severo Ochoa Award of Excellence from MINECO
- MINECO
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Air-stable and readily available Ir-catalyst precursors modified with MaxPHOX-type ligands have been successfully applied in the challenging asymmetric hydrogenation of tetrasubstituted olefins under mild reaction conditions. Gratifyingly, these catalyst precursors are able to efficiently hydrogenate not only a range of indene derivatives (ee's up to 96%) but also 1,2-dihydronapthalene derivatives and acyclic olefins (ee's up to 99%), which both constitute the most challenging substrates for this transformation.
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