Interface Properties of Atomic-Layer-Deposited Al2O3 Thin Films on Ultraviolet/Ozone-Treated Multilayer MoS2 Crystals

We report the interface properties of atomic-layer-deposited Al2O3 thin films on ultraviolet/ozone (UV/O-3)-treated multilayer MoS2 crystals. The formation of S-O bonds on MoS2 after low-power UV/O-3 treatment increased the surface energy, allowing the subsequent deposition of uniform Al2O3 thin films. The capacitance-voltage measurement of Au-Al2O3-MoS2 metal oxide semiconductor capacitors indicated n-type MoS2 with an electron density of similar to 10(17) cm(-3) and a minimum interface trap density of similar to 10(11) cm(-2) eV(-1). These results demonstrate the possibility of forming, a high-quality Al2O3-MoS2 interface by, proper UV/O-3 treatment, providing important implications for their integration into field-effect transistors.