Journal
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
Volume 43, Issue 52, Pages 23319-23326Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2018.10.178
Keywords
Metal-organic frameworks; N-doped CoS2; Nitrogen-doped carbon; Nanosheet arrays; Hydrogen evolution reaction
Categories
Funding
- National Natural Science Foundation of China (NSFC) [51702295, 51702294]
- Natural Science Foundation of Zhejiang [LY18B030004]
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Rational design of highly active, economical and stable electrocatalysts for hydrogen evolution reaction (HER) is still a great challenge for future applications. Herein, we use a 2D metal-organic framework array as the reactive template and precursor, to fabricate a hybrid nanosheet array of nitrogen-rich CoS2@nitrogen-doped carbon on Ti foil substrate (N-CoS2@NC/Ti) through a simple thermal treatment in the presence of thiourea. Owing to the prominent synergistic effect of the coupling between CoS2 and NC, a high content of Co-N-x species as well as unique nanoarray architectures, the as-synthesized N-CoS2@NC/Ti electrode exhibits remarkable activity and robust durability for HER under both acidic and alkaline conditions, which is obviously superior to the CoS2@NC/Ti. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
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