Journal
CATALYSIS TODAY
Volume 342, Issue -, Pages 178-186Publisher
ELSEVIER
DOI: 10.1016/j.cattod.2018.12.005
Keywords
Pincer complex; Ruthenium; Methanol reforming; Hydrogen production; Catalyst immobilization; Supported liquid phase (SLP); Low temperature catalysis
Funding
- German Federal Ministry of Economic Affairs and Energy (BMWi) within the project Metha-Cycle [03ET6071F]
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A homogeneous Ru-pincer complex was immobilized by the supported liquid phase (SLP) technique and tested in continuous gas-phase steam reforming of methanol. Variations of catalyst composition (liquid phase, base and catalyst loading) as well as process parameters (temperature, flow rate) were carried out. High activity was obtained when ionic liquids were used for catalyst immobilization. However, better stability was obtained in the absence of ionic liquids using pure KOH.
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