Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 58, Issue 11, Pages 3279-3284Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201809631
Keywords
electrons; Gibbs energy; insertion; ions; thermodynamics
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Funding
- Deutsche Forschungsgemeinschaft (DFG)
- Ministerio de Economia, Industria y Competitividad (MINECO) [CTQ2017-85317-C2-1-P]
- Fondo Europeo de Desarrollo Regional (ERDF)
- Agencia Estatal de Investigacion (AEI)
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Insertion electrochemical electrodes exhibit simultaneous electron and ion transfer, with the two transfers proceeding across different interfaces. Herein the thermodynamics of the overall electrochemical electrode reaction is discussed with respect to the thermodynamics of these two charge-transfer equilibria. This Minireview includes insertion electrochemical systems where the redox centers are in a solid phase and the ions are transferred between that phase and a solution, and also systems where the redox centers are in a liquid phase that is immiscible with another liquid phase and ions are transferred between the two liquid phases. The Minireview is intended to spark similar studies on battery materials to improve their performance.
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