4.2 Article

Ultra-stable sub-meV monochromator for hard X-rays

Journal

JOURNAL OF SYNCHROTRON RADIATION
Volume 22, Issue -, Pages 1155-1162

Publisher

INT UNION CRYSTALLOGRAPHY
DOI: 10.1107/S1600577515012230

Keywords

high energy-resolution; monochromator; europium; nuclear resonance; cryostat

Funding

  1. US Department of Energy, Basic Energy Sciences, Office of Science [DE-AC02-06CH11357]
  2. National Nuclear Security Administration under Stewardship Science Academic Alliances program through DOE [DE-FC52-06NA27684]

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A high-resolution silicon monochromator suitable for 21.541 keV synchrotron radiation is presented that produces a bandwidth of 0.27 meV. The operating energy corresponds to a nuclear transition in Eu-151. The first-of-its-kind, fully cryogenic design achieves an energy-alignment stability of 0.017 meV r.m.s. per day, or a 100-fold improvement over other meV-monochromators, and can tolerate higher X-ray power loads than room-temperature designs of comparable resolution. This offers the potential for significantly more accurate measurements of lattice excitation energies using nuclear resonant vibrational spectroscopy if combined with accurate energy calibration using, for example, high-speed Doppler shifting. The design of the monochromator along with its performance and impact on transmitted beam properties are presented.

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