Article
Chemistry, Analytical
Yi Xia, Lei Xu, Sufang He, Liexing Zhou, Mingjun Wang, Jing Wang, Sridhar Komarneni
Summary: This study demonstrates the design of an optoelectronic gas sensor based on heterostructures by decorating SnO2 quantum dots on WS2 nanosheets to form 2D/0D structures. The sensor shows fast response/recovery rates and full reversibility to NO2 at room temperature, with enhanced response under ultraviolet illumination.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Chemistry, Analytical
Shang Gao, Yuli Zhao, Wei Wang, Juan Zhao, Xiao Wang
Summary: In this study, an Au decorated CuO/Cu2O composite was synthesized using a water bath method, and it was found that the material exhibited excellent gas sensing performance. The CuO/Cu2O composite showed enhanced response to TEA gas at 160°C, and the response was further improved by Au decoration. The presence of multi-heterojunctions in the materials contributed to their good sensing performance.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Nanoscience & Nanotechnology
Xinzheng Guo, Huachao Yang, Zheng Bo, Jianhua Yan, Kefa Cen
Summary: The study reveals that the optimum interlayer distance of 6-7 angstrom in graphene enhances gas sensor performance and shows increased sensitivity for NO and NO2 at the edge. Multilayer graphene exhibits good selectivity towards NO2, making it a promising candidate for practical low-cost gas sensors.
Review
Chemistry, Multidisciplinary
Zhong Li, Zhengjun Yao, Azhar Ali Haidry, Yange Luan, Yongli Chen, Bao Yue Zhang, Kai Xu, Ruixiang Deng, Nguyen Duc Hoa, Jintang Zhou, Jian Zhen Ou
Summary: The emerging 2D materials have revolutionized various fields and significantly enhanced the performance of physical and chemical sensors. By artificially stacking individual 2D materials to create atomically thin 2D heterostructures, unique features can be realized, leading to improved sensor capabilities.
Review
Chemistry, Analytical
Riya Alice B. John, Karthikeyan Vijayan, Ni Luh Wulan Septiani, Andri Hardiansyah, A. Ruban Kumar, Brian Yuliarto, Angga Hermawan
Summary: This manuscript provides a comprehensive analysis of MXene-based heterostructures in gas-sensing applications. It begins with an overview of gas-sensing mechanisms and explores various features of MXene-based heterostructures, including composites and potential applications. Additionally, engineering strategies are evaluated and compared to other materials in terms of advantages and limitations.
Article
Nanoscience & Nanotechnology
Michal Koci, Tibor Izsak, Gabriel Vanko, Michaela Sojkova, Jana Hrda, Ondrej Szabo, Miroslav Husak, Karol Vegso, Marian Varga, Alexander Kromka
Summary: This study synthesizes MoS2 and H-NCD thin films using appropriate physical/chemical deposition methods, and analyzes their performance in gas sensing properties. The results show that the MoS2/H-NCD heterostructure-based gas sensor exhibits improved sensitivity to oxidizing NO2 and reducing NH3 gases. Different gas interaction model pathways were developed to describe the current flow mechanism through the sensing area.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Analytical
Peng Wang, Tong Song, Guanggang Gao, Katarzyna Matras-Postolek, Ping Yang
Summary: In this study, SnO2 clusters embedded in TiO2 nanosheets were synthesized via a solvothermal method. The gas sensing performance of the resulting heterostructures was significantly enhanced, especially towards acetone, ethanol, and triethylamine, with a response time as short as 10 seconds.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Nanoscience & Nanotechnology
Yanping Chen, Shen Liu, Guiqing Hong, Mengqiang Zou, Bonan Liu, Junxian Luo, Yiping Wang
Summary: This study demonstrates an optomechanical gas pressure sensor based on suspended graphene with ultrahigh sensitivity and a wide range of potential applications.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Multidisciplinary Sciences
Wendong Jia, Chengzhen Hu, Yuqin Wang, Yuming Gu, Guangrui Qian, Xiaoyu Du, Liying Wang, Yao Liu, Jiao Cao, Shanyu Zhang, Shuanghong Yan, Panke Zhang, Jing Ma, Hong-Yuan Chen, Shuo Huang
Summary: The programmable nano-reactors for stochastic sensing (PNRSS) offer a versatile strategy for directly observing various single molecule reactions with refined sensing resolution. This technique can distinguish clinically relevant analogues, such as remdesivir used for treating COVID-19, showing potential applications in pharmacokinetics or drug screening.
NATURE COMMUNICATIONS
(2021)
Article
Nanoscience & Nanotechnology
Muhammad Hamid Raza, Roberto Di Chio, Kaveh Movlaee, Patrick Amsalem, Norbert Koch, Nicolae Barsan, Giovanni Neri, Nicola Pinna
Summary: Heterostructures made from metal oxide semiconductors (MOS) are crucial for high-performance gas sensors. This study explores the transduction mechanism of heterostructured nanomaterials and relates the sensing response to the MOS shell or the p-n heterojunction. The use of carbon nanotubes as conductive substrates enables the devices to operate at low temperature. The findings are important for the development of next generation gas sensing devices.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Nanoscience & Nanotechnology
Mehdi Akbari-Saatlu, Marcin Procek, Claes Mattsson, Goran Thungstrom, Tobias Torndahl, Ben Li, Jiale Su, Wenjuan Xiong, Henry H. Radamson
Summary: Designing heterostructure materials at the nanoscale is a well-known method to enhance gas sensing performance. In this study, ZnO/SnO2 heterostructures were grown on alumina substrates using the ultrasonic spray pyrolysis method. The results showed that the sensitivity of the sensor to H2S gas can be altered by changing the zinc chloride content in the precursor, and the heterostructures with a 5:1 ratio of ZnCl2 to SnCl2·2H(2)O exhibited the highest response. The gas sensing mechanism of the ZnO/SnO2 heterostructures was analyzed and attributed to the formation of the heterostructure between ZnO and SnO2.
ACS APPLIED NANO MATERIALS
(2022)
Article
Chemistry, Analytical
Bharat Sharma, K. Karuppasamy, Ashok Kumar Srivastava, Akram Alfantazi, Ashutosh Sharma
Summary: In this study, boron nitride nanotubes (BNNTs) decorated PtO2 nanoparticles (NPs) were used to form a heterojunction for enhancing the room temperature gas sensing towards dry NH3 gas. The integration of PtO2 NPs onto BNNTs provides a synergistic effect, enabling enhanced NH3 sensing capabilities with low detection limit and short response time, as well as good resistance against humidity and long-term stability.
SENSORS AND ACTUATORS B-CHEMICAL
(2024)
Article
Engineering, Environmental
Huayang Zhu, Xiaohui Liu, Hairui Bai, Tongqing Yang
Summary: Incorporating high permittivity inorganic ferroelectric materials into polymer dielectrics can significantly improve their energy storage capacity. However, the discrepancy in permittivity and the high remnant electric displacement of ferroelectric materials limit the discharged energy density. In this study, a novel nano-heterostructure filler consisting of antiferroelectric nanoparticles (PLSZST) encapsulated with an Al2O3 layer was proposed to alleviate the permittivity discrepancy and enhance the breakdown strength. Experimental and computational results demonstrated that the presence of the Al2O3 layer effectively enhanced the electric displacement and breakdown strength, while reducing the remnant displacement and inhibiting the formation of electrical trees. The nanocomposite films prepared with this filler exhibited impressive discharged energy density and energy storage efficiency near the high electrical breakdown strength, outperforming the current PVDF-based composite dielectrics for high-power energy storage capacitors.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Electrical & Electronic
Akhil Ranjan, Ravikiran Lingaparthi, Nethaji Dharmarasu, K. Radhakrishnan
Summary: This study establishes a theoretical relationship between the properties of a two-dimensional electron gas (2DEG) in AlGaN/GaN HEMT heterostructure and various gas-sensing characteristics. It is proposed that using a thinner barrier layer in the heterostructure can lead to lower detection limits, higher sensing response, and faster response time. Experimental results confirm these analytical findings by comparing a thin-barrier gas sensor with a thick-barrier gas sensor.
IEEE SENSORS JOURNAL
(2022)
Article
Chemistry, Multidisciplinary
Manasi Doshi, Jie Zhang, Eric P. Fahrenthold
Summary: The development of graphene-hBN heterostructures in electronic and gas sensing devices has sparked research interest. Eddy current measurements show lower sheet conductance in graphene-hBN heterostructures compared to previously reported results obtained through contact-based methods. Chemiresistive measurements reveal different incremental sheet conductance responses and sign variations in graphene and graphene-hBN sensors during oxygen adsorption, highlighting the importance of hysteresis in sensing processes.
Article
Materials Science, Multidisciplinary
Steffen Bornemann, Nursidik Yulianto, Hendrik Spende, Yuliati Herbani, Joan Daniel Prades, Hutomo Suryo Wasisto, Andreas Waag
ADVANCED ENGINEERING MATERIALS
(2020)
Article
Chemistry, Analytical
Qomaruddin, Olga Casals, Andris Sutka, Tony Granz, Andreas Waag, Hutomo Suryo Wasisto, Joan Daniel Prades, Cristian Fabrega
Article
Chemistry, Physical
Do Wan Kim, Ki Hong Park, Seung-Hoon Lee, Cristian Fabrega, J. Daniel Prades, Jae-Won Jang
Summary: A highly sensitive and rapidly responsive nitrogen dioxide gas sensor based on gold nanoparticles-decorated zinc oxide nanowires is presented. The study shows that the localized surface plasmon resonance effect of Au NPs can significantly improve the gas response and response time of the sensor.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2021)
Article
Nanoscience & Nanotechnology
K. Kluczyk-Korch, D. Palazzo, A. Waag, A. Dieguez, J. D. Prades, A. Di Carlo, M. Auf der Maur
Summary: This research aims to overcome the spatial resolution limitations of optical systems by developing a spatially resolved light source based on semiconductor nanoLED arrays. Through optical simulations and theoretical analysis, the study explores the design of GaN nanofins and nanorods arrays, finding that suitable array dimensions can improve light output directionality and concentration, potentially leading to chip-based superresolution microscopy with enhanced spatial resolution.
Article
Optics
Hongqiang Li, Sai Zhang, Yikai Zhang, Mingjun Ding, Xinyan Lu, Joan Daniel Prades
Summary: A novel 1550 nm VCSEL based on Group IV elements is proposed, with optimized material composition and quantum well width in the active region. This VCSEL exhibits high coupling efficiency and is a cost-effective, high-yielding and temperature-insensitive on-chip light source suitable for large-scale, high-density monolithic integration.
Article
Chemistry, Analytical
Laura Engel, Ismael Benito-Altamirano, Karina R. Tarantik, Carolin Pannek, Martin Dold, J. Daniel Prades, Juergen Woellenstein
Summary: This study introduces a novel method for monitoring exposure to toxic gases in ambient air using a visible color change in a colorimetric gas sensor. The sensor, made up of a disposable paper tag or plastic card and gas sensitive material deposited by screen-printing, is designed for quantitative evaluation of color change independent of camera and illumination. The colorimetric sensor labels are characterized by the evaluation of RGB values using a smartphone camera at an in-situ readout station.
SENSORS AND ACTUATORS B-CHEMICAL
(2021)
Article
Chemistry, Analytical
Sergio Moreno, Joan Canals, Victor Moro, Nil Franch, Anna Vila, Albert Romano-Rodriguez, Joan Daniel Prades, Daria D. Bershlyakh, Andreas Waag, Katarzyna Kluczyk-Korch, Matthias Auf der Maur, Aldo Di Carlo, Sigurd Krieger, Silvana Geleff, Angel Dieguez
Summary: Recent research on miniaturized illumination sources has led to the development of alternative microscopy techniques, particularly with emerging nano-LED technologies. This research explores the capabilities of nano-LEDs in approaching the optical resolution limit using LED scanning transmission optical microscopy (STOM). The study demonstrates the potential for improving STOM images through oversampling and highlights the possibilities for miniaturized on-chip microscopes using GaN LEDs.
Article
Chemistry, Analytical
Joan Canals, Nil Franch, Victor Moro, Sergio Moreno, Juan Daniel Prades, Albert Romano-Rodriguez, Steffen Bornemann, Dania D. Bershlyakh, Andreas Waag, Florian Vogelbacher, Stefan Schrittwieser, Katarzyna Kluczyk-Korch, Matthias Auf der Maur, Aldo Di Carlo, Angel Dieguez
Summary: The recent advances in chip-size microscopy utilize nano-LEDs to scan samples, achieving high resolution without the need for mechanical parts or optical accessories. Through decreasing LED dimensions in three different implementations, the potential of this new type of microscope is analyzed.
Article
Chemistry, Analytical
Hongqiang Li, Zhixuan An, Shasha Zuo, Wei Zhu, Zhen Zhang, Shanshan Zhang, Cheng Zhang, Wenchao Song, Quanhua Mao, Yuxin Mu, Enbang Li, Juan Daniel Prades Garcia
Summary: This study introduces an artificial intelligence-enabled ECG algorithm based on an improved ResNet for wearable ECG, achieving a classification recognition rate of 98.3% for seven types of arrhythmia signals.
Article
Energy & Fuels
Ugochi Chime, Leon Wolf, Viktoriia Buga, Daniel Weigand, Alaaeldin Gad, Julian Koehler, Andreas Lambertz, Weiyuan Duan, Kaining Ding, Tsvetelina Merdzhanova, Uwe Rau, Oleksandr Astakhov
Summary: Theoretical predictions estimate that thinner silicon wafers may improve efficiency, with open-circuit voltage increasing and fill factor decreasing as wafer thickness decreases. Experimental results show a broad range of high efficiency under 1 sun for wafer thicknesses ranging from 75 to 170 mu m, with the maximum efficiency of 22.3% obtained at 75 mu m. Thinner wafers also show slightly better efficiency at lower light intensity under sun and LED illumination.
Article
Engineering, Electrical & Electronic
Steffen Bornemann, Jan Guelink, Victor Moro, Joan Canals Gil, Stefan Wolter, Georg Schoettler, Daria Bezshlyakh, Joan Daniel Prades, Angel Dieguez, Andreas Waag
Summary: MicroLED arrays can switch each pixel separately with high frequency, making them suitable for various applications. The described scalable chip process chain is used for fabricating passive-matrix microLED arrays with integrated PCB-based driving electronics.
IEEE PHOTONICS JOURNAL
(2021)
Article
Nanoscience & Nanotechnology
Hongqiang Li, Zhixuan An, Sai Zhang, Shasha Zuo, Wei Zhu, Shanshan Zhang, Beiju Huang, Lu Cao, Cheng Zhang, Zanyun Zhang, Wenchao Song, Quanhua Mao, Yuxin Mu, Changyun Miao, Enbang Li, J. Daniel Prades
Summary: The research presented the first fully integrated optical interrogator for the continuous, dynamic, and long-term acquisition of human physiological signals, with the ability to detect body temperature and heart sounds in a wristband. This paves the way for the development of watch-sized integrated wearable optical interrogators with potential applications in health monitoring.
Article
Chemistry, Multidisciplinary
Hongqiang Li, Zhixuan An, Quanhua Mao, Shasha Zuo, Wei Zhu, Shanshan Zhang, Cheng Zhang, Enbang Li, Juan Daniel Prades Garcia
Summary: A waveguide Bragg grating (WBG) has been designed for temperature measurement, with two-sided WBG showing the ability to measure temperature changes within the range of 35-42 degrees Celsius with a measurement error of 0.1 degrees Celsius. This approach has the potential for application in wearable technology and human temperature measurement.
Article
Chemistry, Analytical
Olga Qomaruddin, Olga Casals, Hutomo Suryo Wasisto, Andreas Waag, Joan Daniel Prades, Cristian Fabrega
Summary: This work presents nitrogen dioxide (NO2) gas sensors based on zinc oxide nanorods (ZnO NRs) decorated with gold nanoparticles (Au NPs) that function under visible-light illumination. The study demonstrates the contribution of localized surface plasmon resonant (LSPR) by Au NPs attached to ZnO NRs. The presence of LSPR extends the functionality of ZnO NRs and increases the response at different wavelengths.
Article
Nanoscience & Nanotechnology
Andris Sutka, Raivis Eglitis, Annija Kuzma, Krisjanis Smits, Anzelms Zukuls, Joan Daniel Prades, Cristian Fabrega
Summary: This study demonstrates a gas sensing approach based on photodoping using a thin TiO2 nanoparticle film activated by UV light. The material shows a 1 order of magnitude higher response toward ethanol under UV light compared to no light. This concept enables selective sensor material design.
ACS APPLIED NANO MATERIALS
(2021)
Article
Chemistry, Physical
Sirinya Ukasi, Paritta Jutapukti, Chiranicha Ninthub, Nattapong Pinpru, Phakkhananan Pakawanit, Wanwilai Vittayakorn, Satana Pongampai, Naratip Vittayakorn, Thitirat Charoonsuk
Summary: This study explores the enhancement of electrical output of flexible hybrid piezoelectric-triboelectric nanogenerators by incorporating gamma-glycine into fully organic composites. The research demonstrates the importance of optimized concentrations of gamma-glycine and chitosan in achieving superior performance. The study identifies the critical content of gamma-glycine that leads to the highest output signal, and provides theoretical explanations for this observation.
Article
Chemistry, Physical
Yoonsang Ra, Yu-seop Kim, Seonmo Yang, Namgyu Kang, Gyuwon Oh, Chungyeon Cho, Sangmin Lee, Dongwhi Choi
Summary: In this study, a portable energy harvester (STEP) was proposed to drive various functional LEDs using biomechanical energy. The roles and functionalities of a triboelectric nanogenerator (TENG) and electromagnetic generator (EMG) in the hybrid energy harvester were experimentally demonstrated, and the necessity of hybridization for LED-involved devices was described. The STEP showed promising potential as an effective energy supply strategy for various functional LEDs in related industries.
Article
Chemistry, Physical
Dae Sol Kong, Kyung Hoon Kim, Ying Chieh Hu, Jong Hun Kim, Inseo Kim, Jeongwan Lee, Joonhyuk Lee, Won Hyuk Shon, Hanjin Yoo, Chul-Un Ro, Seungsu Lee, Hyoungjeen Jeen, Minbaek Lee, Minseok Choi, Jong Hoon Jung
Summary: With the rapid development of the Internet of Things and artificial intelligence, smart home has emerged to fulfill the security, convenience, and energy-saving issues of modern life. A flexoelectric mica crystal is used to augment the finger touch-driven triboelectric output for operating a wireless and multichannel smart home controller. This work provides important ingredients for enhancing triboelectric output and realizing a convenient, multifunctional, cost-effective, and adaptable smart home control system without batteries.
Article
Chemistry, Physical
Yi Han, Fang Wu, Xiaozhen Du, Zihao Li, Haixiang Chen, Dongxing Guo, Junlei Wang, Hong Yu
Summary: This paper presents a novel type of triboelectric nanogenerator that utilizes wind energy, with a Y-type bluff body to enhance vibration and output power. The application of this generator successfully provides power for a wireless temperature and humidity sensor.
Article
Chemistry, Physical
Wen Zhang, Fangyuan Cheng, Miao Chang, Yue Xu, Yuyu Li, Shixiong Sun, Liang Wang, Leimin Xu, Qing Li, Chun Fang, Meng Wang, Yuhao Lu, Jiantao Han, Yunhui Huang
Summary: This study successfully induced the formation of a uniform and robust CEI by constructing ZrO2 nano-rivets on the surface of LCO, stabilizing the surface of high-voltage LCO and facilitating lithium-ion diffusion.
Article
Chemistry, Physical
Karl P. Olson, Laurence D. Marks
Summary: This paper investigates the role of contacting shapes in triboelectricity and provides scaling rules for designing energy harvesting devices.
Article
Chemistry, Physical
Jong-An Choi, Jingu Jeong, Mingyu Kang, Hee-Jin Ko, Taehoon Kim, Keun Park, Jongbaeg Kim, Soonjae Pyo
Summary: Wind-driven triboelectric nanogenerators (WTENGs) are a promising emerging technology for sustainable wind energy harvesting, offering high output performance, lightweight design, and compact dimensions. This study introduces an innovative WTENG design that leverages a rolling-based mechanism to achieve efficient omnidirectional wind energy harvesting.
Article
Chemistry, Physical
Liwei Dong, Qian Tang, Chaoyang Zhao, Guobiao Hu, Shuai Qu, Zicheng Liu, Yaowen Yang
Summary: This paper proposes a novel hybrid scheme for flag-type nanogenerators (FNGs) that enhances their performance and broadens their operational wind speed ranges by harnessing the synergistic potential of two aerodynamic behaviors. The proposed flag-type triboelectric-piezoelectric hybrid nanogenerator (FTPNG) integrates flapping piezoelectric flags (PEFs) and a fluttering triboelectric flag (TEF). The FTPNG achieves significant power generation and a broad wind speed range, surpassing other FNGs, making it suitable for various self-powered systems and Internet of Things applications.
Review
Chemistry, Physical
Yunmeng Li, Xin Liu, Zewei Ren, Jianjun Luo, Chi Zhang, Changyong (Chase) Cao, Hua Yuan, Yaokun Pang
Summary: The demand for green and eco-friendly materials is growing due to increasing environmental concerns related to traditional petroleum-based products. Marine biomaterials have emerged as a promising alternative, thanks to their abundant availability, biocompatibility, biodegradability, and low toxicity. In this review, we discuss the development and applications of triboelectric nanogenerators (TENGs) based on marine biomaterials. The operational modes, foundational principles, intrinsic qualities, and advantages of marine biomaterials commonly used in TENG designs are highlighted. Approaches to enhance the efficacy of TENGs derived from marine biomaterials are also discussed, along with documented applications from existing literature. Furthermore, the existing challenges and future directions in marine biomaterial-inspired TENGs are explored.
Article
Chemistry, Physical
Matthew P. Wells, Adam J. Lovett, Yizhi Zhang, Zhongxia Shang, Kosova Kreka, Babak Bakhit, Haiyan Wang, Albert Tarancon, Judith L. MacManus-Driscoll
Summary: Reversible solid oxide cells (rSOCs) offer a promising solution to efficient energy conversion, but have been limited in portable power and electrolysis applications due to excessive polarisation resistance of the oxygen electrode at low temperatures. This study demonstrates the growth of symmetric and complete rSOC structures with reduced polarisation resistance by tuning oxygen vacancy through annealing, providing a promising route towards high-performance rSOC devices for portable power applications.
Article
Chemistry, Physical
Kangkang Bao, Minghui Wang, Yue Zheng, Panpan Wang, Liwen Yang, Yang Jin, Hui Wu, Bin Sun
Summary: This study utilizes ethanol as an electrolyte additive to modulate the migration of zinc ions and the surface structure of zinc anodes, resulting in improved capacity retention and cycle life of zinc-based aqueous batteries.
Article
Chemistry, Physical
Haichao Yang, Wensi Cai, Ming Wang, Saif M. H. Qaid, Zhiyuan Xu, Huaxin Wang
Summary: The introduction of sodium alginate (SA) into perovskite solar cells improves the carrier dynamics, stability, and performance by inhibiting nonradiative recombination and retarded charge dynamics.
Article
Chemistry, Physical
Cuirong Zhang, Mingyuan Wei, Zihan Chen, Wansheng Lin, Shifan Yu, Yijing Xu, Chao Wei, Jinwei Zhang, Ziquan Guo, Yuanjin Zheng, Qingliang Liao, Xinqin Liao, Zhong Chen
Summary: Artificial Intelligence of Things (AIoT) aims to establish smart and informative interactions between humans and devices. However, common pixelated sensing arrays in AIoT applications present problems such as hard and brittle devices, complex structures, and low precision. This article introduces an innovative solution called the all-in-one intelligent semitransparent interactive nerve patch (AISI nerve patch), which integrates sensing, recognition, and transmission functionalities into a thin and flexible patch. The AISI nerve patch is semitransparent, allowing for accurate identification without affecting aesthetics, and it can be attached to any curved surface for intelligent and interactive applications. With rapid response time and high precision recognition, it enables the integration of artificial intelligence and achieves high recognition accuracy for further development of AIoT.
Article
Chemistry, Physical
Youcun Bai, Heng Zhang, Huijun Song, Chong Zhu, Lijin Yan, Qin Hu, Chang Ming Li
Summary: A novel stainless-steel supported lattice-mismatched V-S-Se layered compound with high selenium vacancy was synthesized by adjusting the molar ratio of sulfur to selenium. The introduction of selenium vacancies created additional redox peaks of sulfur, providing more mass transport channels and active sites for zinc ions. The specific capacity and cycle stability of the electrode were significantly improved, demonstrating great potential for practical applications and providing insights into the effects of defects on battery performance.
Article
Chemistry, Physical
Yao Xiao, Puxian Xiong, Yakun Le, Zhenjie Lun, Kang Chen, Zhiduo Wang, Peishan Shao, Zhicong Chen, Dongdan Chen, Zhongmin Yang
Summary: This study successfully synthesized a material with multi-stimulus-responsive luminescence and confirmed the internal relationship between luminescence and defects by regulating the distribution and depth of defects. The dynamic process of multi-stimulus-responsive luminescence was validated by experimental and calculation results.