Article
Chemistry, Multidisciplinary
Yu Zhang, Rana Biswas
Summary: A promising approach to enhance light outcoupling in OLEDs is to utilize internal periodic corrugations that can diffract waveguided and plasmonic modes back to the air cone. Conformally corrugated OLEDs with a photonic crystal substrate exhibit high light outcoupling efficiency around 60-65% and an enhancement factor exceeding 3 for optimal pitch values between 1 and 2.5 μm. Plasmonic losses remain below 10% for all corrugation pitch values, providing a pathway for achieving high light outcoupling over the full optical spectrum.
Article
Optics
Di Yuan, Yaozhen Guo, Bo Liu, Jun Zhao, Zhichao Zhu, Chuanwei Cheng, Hong Chen, Mu Gu, Liang Chen, Jinliang Liu, Xiaoping Ouyang
Summary: This study proposes the use of hollow microlens arrays to enhance the directional light extraction of scintillators, with optical properties conveniently adjusted by varying the microlenses' refractive index and shell thickness. Experimental results are consistent with numerical simulations, indicating the applicability of this scheme to other light-emitting devices with directional emission requirements.
JOURNAL OF LUMINESCENCE
(2021)
Article
Chemistry, Physical
Haotao Li, Fengshou Tian, Shuming Chen
Summary: By synergistically optimizing the optical and electrical performances, the efficiency of quantum-dot light-emitting diodes (QLEDs) can approach the theoretical limit. With the introduction of a high refractive index indium zinc oxide (IZO) electrode and the optimization of its thickness, the light outcoupling efficiency is significantly improved, resulting in an external quantum efficiency (EQE) of 33.2% for red QLEDs. By using a high refractive index plastic substrate and a microlens array, the EQE can be further improved to a record value of 37.5%.
Article
Optics
Bo -Yen Lin, Ya-Xun Lin, Shao-Ju Lin, Yi-Yen Lin, Su-Hua Chen, Mao-Kuo Wei
Summary: The use of self-assembly microlens array films (MAFs) made of silica microspheres and acrylic resin significantly improves the light extraction efficiency (LEE) and angular-spectrum stability of organic light emitting diodes (OLEDs). The MAFs, fabricated through a simple and cost-effective spin-coating process, have a high fill factor of 71.42% and exhibit high transmittance (86.2-90.6%) and high haze (78.9-82.4%) in the UV-Vis regime. The incorporation of MAFs enhances the external quantum efficiency (EQE) of OLEDs by 66% compared to reference OLEDs, while maintaining a small angular shift of CIE-indices and a wide viewing angle range.
JOURNAL OF LUMINESCENCE
(2023)
Article
Optics
Bo-Yen Lin, Yi-Ru Li, Chia-Hsuan Chen, Hao-Chun Hsu, Mao-Kuo Wei, Jiun-Haw Lee, Tien-Lung Chiu
Summary: This study investigates the effects of electron transport layer (ETL) thickness on light extraction in corrugated organic light-emitting diodes (OLEDs). The results show that light extraction in corrugated OLEDs significantly depends on the ETL thickness. Changing the ETL thickness alters the distribution of carrier recombination and results in different attribution of optical loss modes in OLEDs, leading to variations in light extraction and device efficiency.
Article
Optics
Milan Kovacic, Dinara Samigullina, Felix Bouchard, Janez Krc, Benjamin Lipovsek, Marcos Soldera, Andres Fabian Lasagni, Sebastian Reineke, Marko Topic
Summary: Hierarchical textures can enhance the light outcoupling efficiency of OLEDs, and optimization can be achieved by adjusting the aspect ratios of the small and large textures. However, the application of hierarchical textures in laboratory-size samples is constrained by the lateral size of the thin film stack area and the light collection area of the measuring equipment.
Article
Chemistry, Multidisciplinary
Jia Chen, Pingchuan Ma, Wenjing Chen, Zhengguo Xiao
Summary: Photon recycling plays a significant role in increasing the outcoupling efficiency of perovskite light-emitting diodes. Experimental results demonstrate that with the photon recycling effect, the external quantum efficiency (EQE) of PeLEDs can remain above 15%, showing a significant improvement compared to devices without PR.
Article
Chemistry, Multidisciplinary
Jae-Min Kim, Kyu Young Hwang, Sungmin Kim, Junseop Lim, Byungjoon Kang, Kum Hee Lee, Byoungki Choi, Seung-Yeon Kwak, Jun Yeob Lee
Summary: The external quantum efficiency (EQE) of OLEDs can be improved by controlling the light-emitting dipole orientation (EDO) through the design of new phosphorescent materials. This study demonstrates that by modifying the molecular structure of the phosphorescent emitter, the EDO can be effectively enhanced. The results show a linear relationship between EDO and the aspect ratio, and the enhancement of EDO is mainly attributed to the vertical alignment of the molecule's C3 axis.
Article
Materials Science, Multidisciplinary
Yungui Li, Naresh B. Kotadiya, Bas van der Zee, Paul W. M. Blom, Gert-Jan A. H. Wetzelaer
Summary: This study presents a numerical model to simulate the optical outcoupling efficiency of OLEDs with a broad recombination zone, demonstrating that single-layer OLEDs can achieve high outcoupling efficiency similar to multilayer OLEDs. The simulations are validated with experiments on OLEDs of different thickness, showing potential for efficient, stable, and simplified OLED designs.
ADVANCED OPTICAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Wenjing Chen, Jia Chen, Lianghui Gu, Zongming Huang, Pingchuan Ma, Yihan Zhang, Hui Liu, Hongmin Zhou, Nana Wang, Jianpu Wang, Zhengguo Xiao
Summary: The external quantum efficiency of planar-structure perovskite light-emitting diodes (PeLEDs) can be enhanced by forming textured perovskite films. By manipulating the dwell time of antisolvents, the film surface roughness and haze can be controlled, resulting in increased light outcoupling and boosted EQE.
ADVANCED MATERIALS
(2022)
Article
Optics
Guixiong Chen, Yalian Weng, Xiaocong Lai, Wenwen Wang, Xiongtu Zhou, Qun Yan, Tailiang Guo, Yongai Zhang, Chaoxing Wu
Summary: This study successfully improved the light coupling efficiency and angular distribution of OLEDs by designing and integrating hybrid microlens arrays (MLAs) and gratings. By increasing the extraction efficiency with MLAs and improving the angular distribution with gratings, the performance of the OLEDs was enhanced.
Article
Optics
Haotao Li, Shiming Zhou, Shuming Chen
Summary: This study realizes top-emitting quantum-dot light-emitting diodes (QLEDs) with an outcoupling efficiency of over 45% by optimizing the thicknesses of indium-zinc-oxide (IZO) phase tuning layers and IZO top transparent electrodes simultaneously. Moreover, by applying a scattering layer on the IZO top electrode, the red QLEDs show record-breaking efficiencies of EQE 44.5%, power efficiency 92.2 lm W-1, and current efficiency 93.7 cd A(-1).
LASER & PHOTONICS REVIEWS
(2023)
Article
Materials Science, Multidisciplinary
Nils Juergensen, Benjamin Fritz, Adrian Mertens, Jean-Nicolas Tisserant, Mathias Kolle, Guillaume Gomard, Gerardo Hernandez-Sosa
Summary: By integrating light management solutions relying on biodegradable materials in organic light-emitting devices, the development of sustainable light sources or conformable and wearable display technology could be facilitated. Through the utilization of industrially relevant processing techniques, microlens arrays have been seamlessly integrated into flexible and biodegradable cellulose diacetate substrates.
ADVANCED MATERIALS TECHNOLOGIES
(2021)
Review
Chemistry, Physical
Feisong Qin, Min Lu, Po Lu, Siqi Sun, Xue Bai, Yu Zhang
Summary: Perovskite light-emitting diodes (PeLEDs) show great potential for next-generation display and lighting applications due to their excellent optoelectronic properties. However, a systematic overview of the luminescence and degradation mechanisms is currently lacking. This study provides a detailed discussion of the photophysical processes, electroluminescence mechanism, and device degradation of perovskite materials and PeLEDs. Strategies to improve device performances, including optimization of photoluminescence quantum yield, charge injection and recombination, and light outcoupling efficiency, are also summarized. This work aims to guide future development of PeLEDs and facilitate their industrial applications.
Article
Engineering, Electrical & Electronic
Qing Ci, Xingang Ren, Yeqiang Yan, Hao Ren, Kaikun Niu, Guoxing Sun, Zhixiang Huang, Xianliang Wu
Summary: Perovskite light-emitting diodes (PeLEDs) have gained considerable research interest in recent years due to their decent and tunable optoelectronic characteristics. By incorporating nanopatterns, PeLEDs not only exhibit substantial improvement in light extraction intensity, but also reveal remarkable directivity, with the emission angle continuously engineered over 65 degrees. This work is of great importance for engineering highly directional and efficient luminescence devices.
IEEE PHOTONICS JOURNAL
(2021)
Article
Chemistry, Multidisciplinary
Nathan T. Shewmon, Davita L. Watkins, Johan F. Galindo, Raghida Bou Zerdan, Jihua Chen, Jong Keum, Adrian E. Roitberg, Jiangeng Xue, Ronald K. Castellano
ADVANCED FUNCTIONAL MATERIALS
(2015)
Article
Engineering, Electrical & Electronic
Jesse R. Manders, Lei Qian, Alexandre Titov, Jake Hyvonen, Jean Tokarz-Scott, Krishna P. Acharya, Yixing Yang, Weiran Cao, Ying Zheng, Jiangeng Xue, Paul H. Holloway
JOURNAL OF THE SOCIETY FOR INFORMATION DISPLAY
(2015)
Article
Chemistry, Multidisciplinary
Huaibin Shen, Weiran Cao, Nathan T. Shewmon, Chenchen Yang, Lin Song Li, Jiangeng Xue
Article
Optics
Yixing Yang, Ying Zheng, Weiran Cao, Alexandre Titov, Jake Hyvonen, Jesse R. Manders, Jiangeng Xue, Paul H. Holloway, Lei Qian
Article
Materials Science, Multidisciplinary
Xueying Zhao, Davita L. Watkins, Johan F. Galindo, Nathan T. Shewmon, Adrian E. Roitberg, Jiangeng Xue, Ronald K. Castellano, Scott S. Perry
ORGANIC ELECTRONICS
(2015)
Article
Chemistry, Multidisciplinary
Fengjuan Zhang, Shujie Wang, Lei Wang, Qingli Lin, Huaibin Shen, Weiran Cao, Chenchen Yang, Hongzhe Wang, Long Yu, Zuliang Du, Jiangeng Xue, Lin Song Li
Article
Physics, Applied
Daken J. Starkenburg, Paul M. Johns, James E. Baciak, Juan C. Nino, Jiangeng Xue
JOURNAL OF APPLIED PHYSICS
(2017)
Article
Chemistry, Multidisciplinary
Huaibin Shen, Qingli Lin, Weiran Cao, Chenchen Yang, Nathan T. Shewmon, Hongzhe Wang, Jinzhong Niu, Lin Song Li, Jiangeng Xue
Article
Optics
Jing Xie, Jianxiong Bin, Ming Guan, Haikun Liu, Dexin Yang, Jiangeng Xue, Libin Liao, Lefu Mei
JOURNAL OF LUMINESCENCE
(2018)
Article
Materials Science, Multidisciplinary
Asmerom O. Weldeab, April Steen, Daken J. Starkenburg, Jon Steven Dal Williams, Khalil A. Abboud, Jiangeng Xue, Nathan I. Hammer, Ronald K. Castellano, Davita L. Watkins
JOURNAL OF MATERIALS CHEMISTRY C
(2018)
Article
Materials Science, Multidisciplinary
Joshua J. Gabriel, Stephen Xie, Kamal Choudhary, Michael Sexton, Simon R. Phillpot, Jiangeng Xue, Richard G. Hennig
COMPUTATIONAL MATERIALS SCIENCE
(2018)
Article
Physics, Applied
William T. Hammond, John P. Mudrick, Jiangeng Xue
JOURNAL OF APPLIED PHYSICS
(2014)
Article
Chemistry, Physical
Hsien-Yi Hsu, Jarrett H. Vella, Jason D. Myers, Jiangeng Xue, Kirk S. Schanze
JOURNAL OF PHYSICAL CHEMISTRY C
(2014)
Article
Chemistry, Physical
Liang-Jin Xu, Michael Worku, Haoran Lin, Zhengtao Xu, Qingquan He, Chenkun Zhou, Heng Zhang, Yan Xin, Sandrine Lteif, Jiangeng Xue, Biwu Ma
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2019)
Article
Engineering, Electrical & Electronic
James D. Bullock, Zhengtao Xu, Silvano Valandro, Muhammad Younus, Jiangeng Xue, Kirk S. Schanze
ACS APPLIED ELECTRONIC MATERIALS
(2020)