Journal
TETRAHEDRON LETTERS
Volume 49, Issue 11, Pages 1856-1859Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2008.01.023
Keywords
porphyrinoids; benzoporphyrins; magnetic circular dichroism; density functional theory; semiempirical calculations
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A novel low-symmetry tetrabenzoporphine with D-2h symmetry (1) and its zinc complex (2) were prepared via mixed condensation reaction of 5,6-dimethyl phthalimide and 4,5,6,7-tetraphenyl phthalimide with sodium acetate in the presence of zinc acetate. The zinc complex 2 exhibited a split Q band at 640 and 623 nm and a single Soret band at 435 ran. The absorption spectra of I and 2 were calculated and analyzed using Hartree-Fock theory based on INDO/S Hamiltonian. (C) 2008 Elsevier Ltd. All rights reserved.
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