Journal
TETRAHEDRON
Volume 69, Issue 27-28, Pages 5758-5764Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2013.03.011
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Funding
- American Chemical Society [ACS PRF 52119-DNI3]
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We report highly convenient Pd catalysts for the aerobic oxidation of alcohols, which are generated in situ by combining commercially available catalyst precursors. Systematic optimizations of the L- and X-type ligand environment and the employed additive allow the use of air as the sole oxidant without formation of Pd black. The resulting novel protocol provides quantitative yields of a broad variety of ketones and aldehydes. (C) 2013 Elsevier Ltd. All rights reserved.
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