Journal
TETRAHEDRON
Volume 65, Issue 45, Pages 9238-9243Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2009.09.005
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Funding
- Program for Academic Leader in Wuhan Municipality [200851430486]
- National Science Foundation of China [20672040, 20872043]
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An efficient and novel organocatalyst has been developed for the asymmetric desymmetrization of meso- and prochiral ketones by direct Michael addition to nitroolefins. This strategy can afford the desymmetrization products with excellent diastereo- (up to >99:1) and enantioselectivity (up to 96%) in great yields (up to 95%). (C) 2009 Elsevier Ltd. All rights reserved.
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