Journal
TETRAHEDRON
Volume 64, Issue 37, Pages 8815-8829Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2008.06.083
Keywords
labdanes; diterpenes; sclareol
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Funding
- Universidad de Salamanca and to the CICYT [CrQ2005-04406]
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Several 6,7-dioxygenated (cis or trans) labdanes have been synthesised starting front sclareol. A new strategy that allows the obtention of diols alpha-cis as well as beta-cis of trans is described. In particular, the syntheses of three natural highly functionalised labdanes in the B rings of 2, 3 and 4 with different side chains are reported. The syntheses have permitted to Correct the proposed Structure for one of them. (C) 2008 Elsevier Ltd. All rights reserved.
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