Journal
SCRIPTA MATERIALIA
Volume 69, Issue 6, Pages 449-452Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.scriptamat.2013.05.031
Keywords
Nonlinear optical material; Polar structure; Sr3B6O11F2; First-principles calculation
Categories
Funding
- 973 Program of China [2012CB626803]
- National Natural Science Foundation of China [U1129301, 51172277, 21101168, 11104344]
- Main Direction Program of Knowledge Innovation of CAS [KJCX2-EW-H03-03]
- One Hundred Talents Project Foundation Program of CAS
- Funds for Creative Cross & Cooperation Teams of CAS
- Major Program of Xinjiang Uygur Autonomous Region of China [201130111]
- High Technology Research & Development Program of Xinjiang Uygur Autonomous Region of China [201116143]
- Science and Technology Project of Urumqi [G121130002]
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Single crystals of Sr3B6O11F2 were grown using the high-temperature solution method. It produces a second harmonic generation intensity about 2.5 times that of KH2PO4 and is phase-matchable. Its UV cut-off edge is below 190 nm. The complete sets of band structures, birefringence and susceptibility d(ij) coefficients were studied by ab initio calculations. All these properties indicate that Sr3B6O11F2 is a new nonlinear optical crystal applicable in the UV region. Crown Copyright (C) 2013 Published by Elsevier Ltd. on behalf of Acta Materialia Inc. All rights reserved.
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