4.8 Article

Magnetoelastic Excitations in the Pyrochlore Spin Liquid Tb2Ti2O7

Journal

PHYSICAL REVIEW LETTERS
Volume 112, Issue 1, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.112.017203

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Funding

  1. Swiss National Science Foundation [200021_140862]
  2. Swiss National Science Foundation (SNF) [200021_140862] Funding Source: Swiss National Science Foundation (SNF)

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At low temperatures, Tb2Ti2O7 enters a spin liquid state, despite expectations of magnetic order and/or a structural distortion. Using neutron scattering, we have discovered that in this spin liquid state an excited crystal field level is coupled to a transverse acoustic phonon, forming a hybrid excitation. Magnetic and phononlike branches with identical dispersion relations can be identified, and the hybridization vanishes in the paramagnetic state. We suggest that Tb2Ti2O7 is aptly named a magnetoelastic spin liquid and that the hybridization of the excitations suppresses both magnetic ordering and the structural distortion. The spin liquid phase of Tb2Ti2O7 can now be regarded as a Coulomb phase with propagating bosonic spin excitations.

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