4.8 Article

Noninterferometric two-dimensional fourier-transform spectroscopy of multilevel systems

Journal

PHYSICAL REVIEW LETTERS
Volume 100, Issue 22, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.100.227401

Keywords

-

Ask authors/readers for more resources

We demonstrate a technique that determines the phase of the photon-echo emission from spectrally resolved intensity data without requiring phase-stabilized input pulses. The full complex polarization of the emission is determined from spectral intensity measurements. The validity of this technique is demonstrated using simulated data, and is then applied to the analysis of two-color data obtained from the light-harvesting molecule lycopene.

Authors

I am an author on this paper
Click your name to claim this paper and add it to your profile.

Reviews

Primary Rating

4.8
Not enough ratings

Secondary Ratings

Novelty
-
Significance
-
Scientific rigor
-
Rate this paper

Recommended

Article Multidisciplinary Sciences

Persistent coherence of quantum superpositions in an optimally doped cuprate revealed by 2D spectroscopy

Fabio Novelli, Jonathan O. Tollerud, Dharmalingam Prabhakaran, Jeffrey A. Davis

SCIENCE ADVANCES (2020)

Article Optics

Plasmon-induced enhancement of ptychographic phase microscopy via sub-surface nanoaperture arrays

Eugeniu Balaur, Guido A. Cadenazzi, Nicholas Anthony, Alex Spurling, Eric Hanssen, Jacqueline Orian, Keith A. Nugent, Belinda S. Parker, Brian Abbey

Summary: The invention of phase contrast microscopy has enabled the visualization of highly optically transparent samples without the need for staining, revolutionizing optics. Advanced approaches to phase imaging, such as the combination of ptychographic coherent diffractive imaging with plasmonically active metamaterials, have shown significant enhancement in both reconstructed phase and amplitude. This approach opens up new possibilities for imaging a wide range of extremely thin or highly transparent objects previously inaccessible to optical microscopy.

NATURE PHOTONICS (2021)

Article Physics, Multidisciplinary

Many-body effects and quantum fluctuations for discrete time crystals in Bose-Einstein condensates

Jia Wang, Peter Hannaford, Bryan J. Dalton

Summary: A fully comprehensive multi-mode quantum treatment based on truncated Wigner approximation (TWA) was used to study many-body effects and quantum fluctuations on the formation of a discrete time crystal (DTC) in a Bose-Einstein condensate (BEC) bouncing on a periodically driven atom mirror. The study showed that TWA approach can provide accurate predictions and observed the possibility of creating a stable DTC based on repulsive interactions. Additionally, the dynamical behavior of the system was found to be largely independent of whether the boson-boson interaction is attractive or repulsive, indicating the robustness of the system.

NEW JOURNAL OF PHYSICS (2021)

Article Multidisciplinary Sciences

Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor

M. Wurdack, E. Estrecho, S. Todd, T. Yun, M. Pieczarka, S. K. Earl, J. A. Davis, C. Schneider, A. G. Truscott, E. A. Ostrovskaya

Summary: Room-temperature exciton polaritons in a monolayer WS2 exhibit narrow linewidth and enhanced coherence, capable of propagating over tens of micrometers with partial coherence and displaying ballistic transport characteristics. When interacting with cavity photons in optical microcavities, excitons in TMDCs can form exciton polaritons with inherited useful properties.

NATURE COMMUNICATIONS (2021)

Article Biochemical Research Methods

Spectroscopy of excised skin patches exposed to THz and far-IR radiation

Alireza Lajevardipour, Zoltan Vilagosh, Dominique Appadoo, Jeffrey Davis, Saulius Juodkazis, Andrew Wood

Summary: The study found that products containing moisturizing ingredients such as glycerol and sorbitol have significant absorption characteristics in the far-infrared range, while sunscreen ingredients have relatively low absorbance rates. Components like melanin and collagen in dehydrated skin samples also show significant absorption properties, but not as important as moisturizing agents.

BIOMEDICAL OPTICS EXPRESS (2021)

Article Multidisciplinary Sciences

Colorimetric histology using plasmonically active microscope slides

Eugeniu Balaur, Sandra O' Toole, Alex J. Spurling, G. Bruce Mann, Belinda Yeo, Kate Harvey, Catherine Sadatnajafi, Eric Hanssen, Jacqueline Orian, Keith A. Nugent, Belinda S. Parker, Brian Abbey

Summary: This study demonstrates the generation of colorimetric histology images using full-sized plasmonically active microscope slides. These slides translate subtle changes in dielectric constant into striking color contrast when samples are placed on them. The biomedical potential of this technique is shown by distinguishing neoplastic cells from normal breast epithelium in mouse models and in human diagnostic tissue. Comparing the colorimetric output with conventional histopathology shows the potential for histoplasmonics as an alternative or adjunct to staining.

NATURE (2021)

Article Materials Science, Multidisciplinary

Direct measurement of biexcitons in monolayer WS2

M. A. Conway, J. B. Muir, S. K. Earl, M. Wurdack, R. Mishra, J. O. Tollerud, J. A. Davis

Summary: This study successfully identifies and separates the optically excited biexciton in monolayer WS2 using two-quantum multidimensional coherent spectroscopy (2Q-MDCS), and measures the binding energy of the biexciton. The biexciton is composed of two bright excitons in opposite valleys.

2D MATERIALS (2022)

Correction Multidisciplinary Sciences

Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor (vol 12, 5366, 2021)

M. Wurdack, E. Estrecho, S. Todd, T. Yun, M. Pieczarka, S. K. Earl, J. A. Davis, C. Schneider, A. G. Truscott, E. A. Ostrovskaya

NATURE COMMUNICATIONS (2022)

Article Multidisciplinary Sciences

Megahertz pulse trains enable multi-hit serial femtosecond crystallography experiments at X-ray free electron lasers

Susannah Holmes, Henry J. Kirkwood, Richard Bean, Klaus Giewekemeyer, Andrew Martin, Marjan Hadian-Jazi, Max O. Wiedorn, Dominik Oberthuer, Hugh Marman, Luigi Adriano, Nasser Al-Qudami, Sasa Bajt, Imrich Barak, Sadia Bari, Johan Bielecki, Sandor Brockhauser, Mathew A. Coleman, Francisco Cruz-Mazo, Cyril Danilevski, Katerina Doerner, Alfonso M. Ganan-Calvo, Rita Graceffa, Hans Fanghor, Michael Heymann, Matthias Frank, Alexander Kaukher, Yoonhee Kim, Bostjan Kobe, Juraj Knoska, Torsten Laurus, Romain Letrun, Luis Maia, Marc Messerschmidt, Markus Metz, Thomas Michelat, Grant Mills, Serguei Molodtsov, Diana C. F. Monteiro, Andrew J. Morgan, Astrid Muennich, Gisel E. Pena Murillo, Gianpietro Previtali, Adam Round, Tokushi Sato, Robin Schubert, Joachim Schulz, Megan Shelby, Carolin Seuring, Jonas A. Sellberg, Marcin Sikorski, Alessandro Silenzi, Stephan Stern, Jola Sztuk-Dambietz, Janusz Szuba, Martin Trebbin, Patrick Vagovic, Thomas Ve, Britta Weinhausen, Krzysztof Wrona, Paul Lourdu Xavier, Chen Xu, Oleksandr Yefanov, Keith A. Nugent, Henry N. Chapman, Adrian P. Mancuso, Anton Barty, Brian Abbey, Connie Darmanin

Summary: The European XFEL MHz SFX technique enables tracking of sub-microsecond structural changes in individual crystals, allowing for multi-hit serial crystallography. This technique overcomes the issue of radiation damage in traditional methods.

NATURE COMMUNICATIONS (2022)

Article Engineering, Electrical & Electronic

Comparison of supercontinuum generation spectral intensity in benzene-core PCFs with different types of lattices in the claddings

L. Chu Van, B. T. Le Tran, T. Nguyen Thi, D. Hoang Trong, T. Dang Van, T. Do Mai, H. Trinh Ngoc, T. Thai Doan, K. Doan Quoc

Summary: This article investigates the nonlinear characteristics of three newly designed benzene-core photonic crystal fibers and selects the optimal fiber structure. The results demonstrate that these fibers are highly efficient for supercontinuum generation.

OPTICAL AND QUANTUM ELECTRONICS (2022)

Article Multidisciplinary Sciences

Interactions between Fermi polarons in monolayer WS2

Jack B. Muir, Jesper Levinsen, Stuart K. Earl, Mitchell A. Conway, Jared H. Cole, Matthias Wurdack, Rishabh Mishra, David J. Ing, Eliezer Estrecho, Yuerui Lu, Dmitry K. Efimkin, Jonathan O. Tollerud, Elena A. Ostrovskaya, Meera M. Parish, Jeffrey A. Davis

Summary: Researchers introduced mobile exciton impurities into a two-dimensional electron gas and conducted experiments on monolayer WS2 using multi-dimensional coherent spectroscopy. They found that at low electron doping densities, the dominant interactions occur between polaron states dressed by the same Fermi sea. Additionally, they discovered a bipolaron bound state with remarkably large binding energy involving excitons in different valleys cooperatively bound to the same electron.

NATURE COMMUNICATIONS (2022)

Article Optics

Broadband supercontinuum generation in cascaded tapered liquid core fiber

Lanh Chu Van, Ngoc Vo Thi Minh, Bao Tran Le Tran, Trong Dang Van, Phuong Nguyen Thi Hong, Trang Do Mai, Trung Le Canh, Hieu Van Le, Thuy Nguyen Thi, Thanh Thai Doan, Van Thuy Hoang

Summary: This article investigates the use of tapered liquid-core fibers for supercontinuum generation through numerical simulations. The results show that tapered fibers have the potential for high coupling efficiency and high nonlinearity. By changing the core diameter, both all-normal dispersion and anomalous dispersion supercontinuum generation can be achieved. Furthermore, the use of cascaded tapered fibers can mitigate thermal effects and increase the stability of the output supercontinuum spectra.

OPTICS COMMUNICATIONS (2023)

Article Chemistry, Multidisciplinary

Effects of Floquet Engineering on the Coherent Exciton Dynamics in Monolayer WS2

Mitchell A. Conway, Stuart K. Earl, Jack B. Muir, Thi-Hai-Yen Vu, Jonathan O. Tollerud, Kenji Watanabe, Takashi Taniguchi, Michael S. Fuhrer, Mark T. Edmonds, Jeffrey A. Davis

Summary: By using multidimensional coherent spectroscopy, we excited, controlled, and probed a coherent superposition of excitons in the K and K' valleys in monolayer WS(2). We observed phase rotations greater than π and showed that this could be described by a combination of the AC-Stark shift and the Bloch-Siegert shift. However, the process was not perfectly adiabatic and additional decoherence caused by power broadening was observed. These nonadiabatic effects may pose problems for certain applications, but the measurements also suggest ways to minimize or eliminate them.

ACS NANO (2023)

Article Materials Science, Multidisciplinary

Coherent dynamics of Floquet-Bloch states in monolayer WS2 reveals fast adiabatic switching

S. K. Earl, M. A. Conway, J. B. Muir, M. Wurdack, E. A. Ostrovskaya, J. O. Tollerud, J. A. Davis

Summary: The research team used femtosecond laser pulses to demonstrate the optical Stark effect in monolayer WS2, showing adiabatic evolution of the system and linear dependence of induced energy shift on instantaneous intensity, even for ultrafast driving fields of fewer than 15 optical cycles.

PHYSICAL REVIEW B (2021)

Article Computer Science, Artificial Intelligence

Multidimensional analysis of excitonic spectra of monolayers of tungsten disulphide: toward computer-aided identification of structural and environmental perturbations of 2D materials

Pavel Kolesnichenko, Qianhui Zhang, Changxi Zheng, Michael S. Fuhrer, Jeffrey A. Davis

Summary: Despite the great promise of 2D materials for various applications, the reality of device proliferation and meeting real-life demands is still far from being achieved. Experimentally obtainable samples commonly experience a wide range of perturbations that significantly deviate the properties from idealistic models, making it challenging for physical property interpretations and disentanglement of effects. Through statistical correlation analysis and unsupervised machine learning algorithms, we can identify dominant components related to tensile strain, disorder induced by environmental molecules, multi-layer regions, and charge doping, in excitonic spectra of WS2 monolayers. This approach has the potential to determine the local environment of 2D materials and pave the way for advanced, machine-aided characterization of monolayer matter.

MACHINE LEARNING-SCIENCE AND TECHNOLOGY (2021)

No Data Available