4.6 Article

Plasmon bands in multilayer graphene

Journal

PHYSICAL REVIEW B
Volume 90, Issue 23, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.90.235434

Keywords

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Funding

  1. German Research Foundation (DFG)
  2. Ministry of Science, Research and Arts (MWK) of the state Baden-Wurttemberg within the Sub-Angstrom Low-Voltage Electron Microscopy project (SALVE)

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High-energy collective electronic excitations (plasmons) in freestanding multilayer graphene are studied by momentum-resolved electron energy-loss spectroscopy (EELS). For normal incidence, only the high-energy plasmon band is excited and we measure a blueshift of the pi-plasmon dispersion with increasing thickness. The observed transition between two-dimensional and three-dimensional behavior is explained using a layered-electron-gas (LEG) model. We propose a method to measure all individual plasmon bands by tilting the sample with respect to the electron beam. As a proof of concept, EELS experiments for three-layer graphene are compared with predictions from the LEG model.

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