Article
Materials Science, Multidisciplinary
Biplab Bag, Sourav M. Karan, Gorky Shaw, A. K. Sood, A. K. Grover, S. S. Banerjee
Summary: Time series measurements in 2H-NbS2 crystal have revealed a drive-induced transition from low to high critical current jammed vortex state via negative differential resistance (NDR) transition. The probability of observing the NDR transition increases systematically with magnetic field in weak collective pinning regime and becomes field independent in strong pinning regime. The NDR transition occurs in a high dissipation regime, leading to a high entropy vortex state with high critical current.
Article
Materials Science, Multidisciplinary
Maria Jose Cortes Burgos, Pamela C. Guruciaga, Daniel Jordan, Cynthia P. Quinteros, Elisabeth Agoritsas, Javier Curiale, Mara Granada, Sebastian Bustingorry
Summary: The study investigates the creep motion of domain walls in magnetic thin films driven by external fields and discusses the roughness exponent and amplitude, with experimental results showing an average roughness exponent value of 0.74 and a significant increase in roughness amplitude with decreasing field intensity. These results contribute to understanding domain wall motion in disordered magnetic thin systems.
Article
Physics, Multidisciplinary
Jiaruo Li, Oleg Yu Gorobtsov, Sheena K. K. Patel, Nelson Hua, Benjamin Gregory, Anatoly G. Shabalin, Stjepan Hrkac, James Wingert, Devin Cela, James M. Glownia, Matthieu Chollet, Diling Zhu, Rajasekhar Medapalli, Eric E. Fullerton, Oleg G. Shpyrko, Andrej Singer
Summary: This study demonstrates experimentally the role phonons play in SDW formation after an SDW-quench by femtosecond laser pulses. The temperature-dependent SDW period in thin films is quantized, allowing for precise tracking of the out-of-equilibrium formation path of the SDW.
COMMUNICATIONS PHYSICS
(2022)
Article
Physics, Multidisciplinary
Francesco Petocchi, Christopher W. Nicholson, Bjoern Salzmann, Diego Pasquier, Oleg Yazyev, Claude Monney, Philipp Werner
Summary: We address the problem of the ground state of 1T-TaS2 by studying the correlated electronic structure of stacked bilayers. The surface termination determines whether the uncorrelated system is band insulating or exhibits a metallic surface state. A Mott gap opens in the surface state but is smaller than the gap originating from the bilayer structure. Our results are consistent with recent experimental measurements and clarify the interplay between Mott insulating and band insulating behavior in this system.
PHYSICAL REVIEW LETTERS
(2022)
Article
Materials Science, Multidisciplinary
Li Cheng, Xuanyu Long, Xiaobin Chen, Xiaolong Zou, Zheng Liu
Summary: The study shows that a flat band in 1T-TaS2 can be understood by adjusting the t(2g) basis, and the rehybridization of three orbitals by the CDW order leads to the formation of the flat band.
Article
Multidisciplinary Sciences
Sangjun Lee, Edwin W. Huang, Thomas A. Johnson, Xuefei Guo, Ali A. Husain, Matteo Mitrano, Kannan Lu, Alexander Zakrzewski, Gilberto A. de la Pena, Yingying Peng, Hai Huang, Sang-Jun Lee, Hoyoung Jang, Jun-Sik Lee, Young Il Joe, William B. Doriese, Paul Szypryt, Daniel S. Swetz, Songxue Chi, Adam A. Aczel, Gregory J. MacDougall, Steven A. Kivelson, Eduardo Fradkin, Peter Abbamonte
Summary: The behavior of charge density waves (CDWs) in different families of copper-oxide superconductors has been studied. This research found that the CDW amplitude is temperature independent and develops well above experimentally accessible temperatures. The CDW wavevector shows a nonmonotonic temperature dependence, exhibiting different behaviors at low temperatures and near the spin ordering temperature. The study suggests a common mechanism for CDW order in all families of cuprates.
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2022)
Article
Materials Science, Multidisciplinary
Jingwei Dong, Weiyan Qi, Dongbin Shin, Laurent Cario, Zhesheng Chen, Romain Grasset, Davide Boschetto, Mateusz Weis, Pierrick Lample, Ernest Pastor, Tobias Ritschel, Marino Marsi, Amina Taleb, Noejung Park, Angel Rubio, Evangelos Papalazarou, Luca Perfetti
Summary: This study compares the bulk and surface properties of the transition metal dichalcogenide 1T-TaS2. It is found that when heating the sample, the surface exhibits an intermediate insulating phase while the bulk remains metallic. The amplitude mode at the surface is always stiffer and shows variable coupling to the Mott-Peierls band in different phases.
Article
Materials Science, Multidisciplinary
Lukas Schwarz, Rafael Haenel, Dirk Manske
Summary: This paper introduces the use of THG experiments on superconductors to study collective excitations like the Higgs mode, and additionally analyzes the phase of the THG signal for the first time, highlighting the importance of phase information in interpreting experimental results.
Article
Multidisciplinary Sciences
Huimin Zhang, Basu Dev Oli, Qiang Zou, Xu Guo, Zhengfei Wang, Lian Li
Summary: In FeSn, we observe the symemtry-breaking and tunable electronic orders in the Kagome lattice by applying a magnetic field, providing a new avenue for studying the unique quantum states in Kagome lattice.
NATURE COMMUNICATIONS
(2023)
Article
Physics, Multidisciplinary
Zhengxin Wei, Shuai Zhang, Yulun Su, Liang Cheng, Haidong Zhou, Zhigang Jiang, Hongming Weng, Jingbo Qi
Summary: In this study, we investigated the dynamics of quasiparticles and collective excitations in the material ZrTe5 using ultrafast optical pump-probe spectroscopy. Our results revealed two coherent oscillations with extremely low energies, which softened as the temperature approached two different critical temperatures. These oscillations were attributed to the amplitude mode of photoinduced dynamic charge density waves in ZrTe5. Additionally, we observed a peculiar quasiparticle decay process associated with a specific mode below a transition temperature. These findings provide important information for studying fluctuating order parameters and quasiparticle dynamics in different low-dimensional topological systems and materials.
SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY
(2022)
Article
Multidisciplinary Sciences
Shiwei Shen, Chenhaoping Wen, Pengfei Kong, Jingjing Gao, Jianguo Si, Xuan Luo, Wenjian Lu, Yuping Sun, Gang Chen, Shichao Yan
Summary: Researchers demonstrate a transition from an insulating gap to a tunable Kondo resonance in 1T-TaS2 by Pb intercalation, providing a pathway for creating and tuning many-body electronic states in layered narrow-electronic-band materials.
NATURE COMMUNICATIONS
(2022)
Article
Physics, Multidisciplinary
Wei Ruan, Yi Chen, Shujie Tang, Jinwoong Hwang, Hsin-Zon Tsai, Ryan L. Lee, Meng Wu, Hyejin Ryu, Salman Kahn, Franklin Liou, Caihong Jia, Andrew Aikawa, Choongyu Hwang, Feng Wang, Yongseong Choi, Steven G. Louie, Patrick A. Lee, Zhi-Xun Shen, Sung-Kwan Mo, Michael F. Crommie
Summary: Research has shown that some quantum spin liquids may have an effective Fermi surface of fractionalized spinon excitations. The material 1T-TaSe2 is believed to have charge density modulations caused by an unstable spinon Fermi surface. Through scanning tunnelling spectroscopy, researchers have imaged density waves consistent with the predictions of spinon density modulation in single-layer 1T-TaSe2. Additionally, spectroscopic imaging of isolated single-layer 1T-TaSe2 has revealed long-wavelength super-modulations consistent with the behavior of itinerant spinons, allowing the experimental measurement of the spinon Fermi wavevector.
Article
Chemistry, Multidisciplinary
Hossain Mohammad Ikram, Ara Ferdous, Shahed Syed Mohammad Fakruddin, Zhipeng Wang, Tadahiro Komeda
Summary: We report the finding of a 1T phase island of NbSe2 on a cleaved surface and its magnetic properties. The magnetic moment placed in the superconducting state generates the Yu-Shiba-Rusinov (YSR) state with specific position and anisotropic decay behavior. The enhancement of the YSR peak is closely related to the local curvature of the film.
Article
Materials Science, Multidisciplinary
Grace P. Chen, Elena Bykova, Maxim Bykov, Eric Edmund, Zi-Yu Cao, Xiao-Jia Chen, Jesse S. Smith, Stella Chariton, Vitali B. Prakapenka, Alexander F. Goncharov
Summary: The high-pressure properties of layered transition metal dichalcogenide 2H-NbSe2 were investigated, revealing its structural stability up to 35 GPa. The lattice compressibility changes from anisotropic to isotropic with increasing pressure. The compression behavior of interatomic bonds is highly anisotropic, while the intramolecular bonds show a nonmonotonic pressure dependence with a maximum at -12 GPa.
Article
Nanoscience & Nanotechnology
Gan Liu, Tianyu Qiu, Kuanyu He, Yizhou Liu, Dongjing Lin, Zhen Ma, Zhentao Huang, Wenna Tang, Jie Xu, Kenji Watanabe, Takashi Taniguchi, Libo Gao, Jinsheng Wen, Jun-Ming Liu, Binghai Yan, Xiaoxiang Xi
Summary: In this study, electrical switching of ferro-rotational domain states in the charge-density-wave phases of nanometre-thick 1T-TaS2 crystals is demonstrated. Despite the lack of coupling between the electric field and the ferroic order due to symmetry mismatch, the electric field drives domain wall propagation, resulting in reversible, durable, and non-volatile isothermal state switching.
NATURE NANOTECHNOLOGY
(2023)
Review
Chemistry, Multidisciplinary
Seungbum Hong, Chi Hao Liow, Jong Min Yuk, Hye Ryung Byon, Yongsoo Yang, EunAe Cho, Jiwon Yeom, Gun Park, Hyeonmuk Kang, Seunggu Kim, Yoonsu Shim, Moony Na, Chaehwa Jeong, Gyuseong Hwang, Hongjun Kim, Hoon Kim, Seongmun Eom, Seongwoo Cho, Hosun Jun, Yongju Lee, Arthur Baucour, Kihoon Bang, Myungjoon Kim, Seokjung Yun, Jeongjae Ryu, Youngjoon Han, Albina Jetybayeva, Pyuck-Pa Choi, Joshua C. Agar, Sergei Kalinin, Peter W. Voorhees, Peter Littlewood, Hyuck Mo Lee
Summary: Multiscale and multimodal imaging of material structures and properties provide a solid foundation for materials theory and design to flourish. The M3I3 initiative aims to reduce time for the discovery, design and development of materials based on quantifying and understanding multiscale processing-structure-property relationships. By combining machine learning and scientific insights, the vision of M3I3 can be realized through elucidating these relationships and material hierarchies.
Article
Materials Science, Multidisciplinary
Alejandro Lopez-Bezanilla, Peter B. Littlewood
Summary: An insulating-metallic transition is predicted in a series of two-dimensional carbon-based structures mediated by substitutional atoms. Introducing Si atoms at selected sites and maintaining metallic properties accurately by BN dimers, a series of isomorphous two-dimensional materials with various band gaps is created.
PHYSICAL REVIEW MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Alejandro Lopez-Bezanilla, Peter B. Littlewood
Summary: In a hollow structure with both thermal and dynamical stability, excellent photovoltaic performance is predicted for a pentagonal covalent network of Si, characterized by a combination of sp(2) and sp(3) hybridized Si atomic orbitals. The computed band structure shows an indirect band gap near the zone edge and directly absorbing transitions at visible light frequencies, suggesting the possibility of obtaining a stable phase with low formation energy under low pressure conditions.
Article
Multidisciplinary Sciences
Michel Fruchart, Ryo Hanai, Peter B. Littlewood, Vincenzo Vitelli
Summary: The article discusses the impact of non-reciprocity on the collective behavior of multi-body systems in out-of-equilibrium states, indicating that non-reciprocity leads to the emergence of time-dependent phases controlled by exceptional points. The article describes the non-reciprocal generalizations of three archetypal classes of self-organization out of equilibrium, including synchronization, flocking, and pattern formation.
Article
Chemistry, Physical
Edoardo Fertitta, Sujit Das, Debalina Banerjee, Farbod Ebrahimi, Clement Barraud, Kai Du, He Tian, Chris J. Pickard, Cedric Weber, Ramamoorthy Ramesh, Peter Littlewood, David Dubbink
Summary: The study focuses on the characterization of double perovskite oxides La2TiFeO6 and La2VCuO6, exploring B-site disorder and partial charge transfer between B-site ions. Utilizing random structure sampling method, multiple phases competing due to their configurational entropy were identified. Evaluation of information encapsulated in potential energy landscape via structure sampling optimized the metric for competition of different phases.
NPJ COMPUTATIONAL MATERIALS
(2021)
Article
Physics, Condensed Matter
Laura E. Ratcliff, Luigi Genovese, Hyowon Park, Peter B. Littlewood, Alejandro Lopez-Bezanilla
Summary: This study provides a detailed exploration of the f-atomic orbital occupancy space for UO2 using a first principles approach based on density functional theory. The results show that the computational complexity of the energy landscape of a correlated f-electron oxide is much richer than previously demonstrated, and multiple previously unexplored metastable electronic states of UO2 have been discovered.
JOURNAL OF PHYSICS-CONDENSED MATTER
(2022)
Article
Materials Science, Multidisciplinary
Menglu Chen, Xinzheng Lan, Margaret H. Hudson, Guohua Shen, Peter B. Littlewood, Dmitri Talapin, Philippe Guyot-Sionnest
Summary: The magnetoresistance of HgTe quantum dot films shows a positive-quadratic effect correlated with the filling fraction and a negative exponential effect independent of the fractional occupation.
JOURNAL OF MATERIALS CHEMISTRY C
(2022)
Article
Physics, Multidisciplinary
Bipul Pandey, Peter B. Littlewood
Summary: In the context of a single-electron two orbital Holstein system coupled to dispersionless bosons, a general method to correct the single-particle Green's function using a power series correction (PSC) scheme is developed. The derivations and assumptions behind various flavors of cumulant approximation through the PSC scheme are outlined. Comparisons between the PSC spectral function, cumulant, and exact diagonalized spectral functions reveal three regimes, two of which can be explained by the cumulant approximation and one where it fails. It is found that the exact and PSC spectral functions match within spectral broadening across all three regimes.
PHYSICAL REVIEW LETTERS
(2022)
Article
Energy & Fuels
Gavin D. J. Harper, Emma Kendrick, Paul A. Anderson, Wojciech Mrozik, Paul Christensen, Simon Lambert, David Greenwood, Prodip K. Das, Mohamed Ahmeid, Zoran Milojevic, Wenjia Du, Dan J. L. Brett, Paul R. Shearing, Alireza Rastegarpanah, Rustam Stolkin, Roberto Sommerville, Anton Zorin, Jessica L. Durham, Andrew P. Abbott, Dana Thompson, Nigel D. Browning, B. Layla Mehdi, Mounib Bahri, Felipe Schanider-Tontini, D. Nicholls, Christin Stallmeister, Bernd Friedrich, Marcus Sommerfeld, Laura L. Driscoll, Abbey Jarvis, Emily C. Giles, Peter R. Slater, Virginia Echavarri-Bravo, Giovanni Maddalena, Louise E. Horsfall, Linda Gaines, Qiang Dai, Shiva J. Jethwa, Albert L. Lipson, Gary A. Leeke, Thomas Cowell, Joseph Gresle Farthing, Greta Mariani, Amy Smith, Zubera Iqbal, Rabeeh Golmohammadzadeh, Luke Sweeney, Vannessa Goodship, Zheng Li, Jacqueline Edge, Laura Lander, Viet Tien Nguyen, Robert J. R. Elliot, Oliver Heidrich, Margaret Slattery, Daniel Reed, Jyoti Ahuja, Aleksandra Cavoski, Robert Lee, Elizabeth Driscoll, Jen Baker, Peter Littlewood, Iain Styles, Sampriti Mahanty, Frank Boons
Summary: This roadmap presents the market dynamics and their influence on a future circular economy for lithium-ion batteries (LIB), with a focus on safety throughout the life cycle. Various options for end-of-life (EOL) disposal, such as remanufacturing, reuse, and recycling, are discussed. Diagnostics play a crucial role in assessing battery health and condition, and improvements to diagnostic techniques are evaluated. The future of LIB recycling lies in automated dismantling of EOL battery packs and the development of design for recycling and new cell design approaches.
JOURNAL OF PHYSICS-ENERGY
(2023)
Article
Chemistry, Physical
Simon A. J. Kimber, Jiayong Zhang, Charles H. Liang, Gian G. Guzman-Verri, Peter B. Littlewood, Yongqiang Cheng, Douglas L. Abernathy, Jessica M. Hudspeth, Zhong-Zhen Luo, Mercouri G. Kanatzidis, Tapan Chatterji, Anibal J. Ramirez-Cuesta, Simon J. L. Billinge
Summary: Using the energy-resolved variable-shutter pair distribution function technique, we found that GeTe materials at higher temperatures exhibit anisotropic and non-linear dynamics, resembling static disorder. Our Ginzburg-Landau model coupling polarization fluctuations explains the emergence of this anisotropy. By studying the time-dependent atomic correlations in energy materials, we reconcile the long-standing disagreement between local and average structure probes and demonstrate the ubiquity of spontaneous anisotropy in cubic IV-VI materials.
Article
Physics, Multidisciplinary
G. G. Guzman-Verri, C. H. Liang
Summary: We used the self-consistent phonon approximation to investigate the effects of flexoelectric interaction on ferroelectric materials and found that long-range modulated order is unstable at all temperatures. This study has important implications for nearly ferroelectric materials such as SrTiO3 and KTaO3, and suggests that these materials may be melted versions of an underlying modulated state dominated by nonzero momentum thermal fluctuations.
PHYSICAL REVIEW LETTERS
(2023)
Article
Biotechnology & Applied Microbiology
Jonathan A. Poli, Christopher Howard, Alfredo J. Garcia, Don Remboski, Peter B. Littlewood, John P. Kress, Narayanan Kasthuri, Alia Comai, Kiran Soni, Philip Kennedy, John Ogger, Robert M. DiBlasi
Summary: The COVID-19 pandemic has highlighted the need for effective respiratory support in healthcare settings. This report introduces a novel 3D-printed valve system called BubbleVent that can provide intermittent mandatory ventilation for adult patients without direct electrification. Testing shows that BubbleVent can deliver stable pressure levels and comparable breath timing control with a critical care ventilator.
BIOENGINEERING-BASEL
(2022)
Article
Materials Science, Multidisciplinary
Mark Steger, Ryo Hanai, Alexander Orson Edelman, Peter B. Littlewood, David W. Snoke, Jonathan Beaumariage, Brian Fluegel, Ken West, Loren N. Pfeiffer, Angelo Mascarenhas
Summary: The researchers observed the existence of the Higgs amplitude mode in exciton-polariton condensates, driven purely by intrinsic quantum fluctuations instead of perturbations. They used an ultrahigh quality microcavity and a Raman spectrometer to reject photoluminescence and observed spectral features in good agreement with their theoretical analysis.
Article
Physics, Multidisciplinary
Ryo Hanai, Peter B. Littlewood
PHYSICAL REVIEW RESEARCH
(2020)
Article
Materials Science, Multidisciplinary
L. Shen, S. A. Mack, G. Dakovski, G. Coslovich, O. Krupin, M. Hoffmann, S-W Huang, Y-D Chuang, J. A. Johnson, S. Lieu, S. Zohar, C. Ford, M. Kozina, W. Schlotter, M. P. Minitti, J. Fujioka, R. Moore, W-S Lee, Z. Hussain, Y. Tokura, P. Littlewood, J. J. Turner