Journal
PHYSICAL REVIEW B
Volume 88, Issue 1, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.88.014504
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Funding
- European Commission under the 6th Framework Programme through the Key Action: Strengthening the European Research Area, Research Infrastructures [RII3-CT-2003-505925 (NMI3)]
- Indo-Swiss Joint Research Program (ISJRP) by Swiss State Secretariat of Education and Research [JRP122960]
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The spin-gap evolution upon Ca doping in Sr14-xCaxCu24O41 was systematically investigated using inelastic neutron scattering. We discover that the singlet-triplet spin-gap excitation survives in this series with x up to 13, indicating the singlet dimer ground state in these compounds. This observation corrects the previous speculation that the spin gap collapses at x similar to 13 by the NMR technique. The strong intensity modulation along Q(H) in x = 0 gradually evolves into a Q-independent feature in x > 11. This could be attributed to the localized Cu moment magnetism developing into an itinerant magnetism with increasing x. It is a surprise that the spin gap persists in the normal state of this spin-ladder system with metallic behavior, which evidences the possibility of magnetically mediated carrier pairing mechanism in a two-leg spin-ladder lattice.
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