Journal
PHYSICAL REVIEW B
Volume 80, Issue 22, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.80.220409
Keywords
band structure; charge-ordered states; electronic density of states; ferrimagnetic materials; ferroelectric materials; ground states; lutetium compounds; magnetic moments; magnetoelectric effects; multiferroics; X-ray emission spectra; X-ray photoelectron spectra
Funding
- Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, USA [DE-AC03-76SF00098]
- Lichtenberg program of the Federal State of Lower Saxony
- [GRK695]
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Electronic and magnetic properties of the charge ordered phase of LuFe2O4 are investigated by means of x-ray spectroscopic and theoretical electronic structure approaches. LuFe2O4 is a compound showing fascinating magnetoelectric coupling via charge ordering. Here, we identify the spin ground state of LuFe2O4 in the charge ordered phase to be a 2:1 ferrimagnetic configuration, ruling out a frustrated magnetic state. An enhanced orbital moment may enhance the magnetoelectric coupling. Furthermore, we determine the densities of states and the corresponding correlation potentials by means of x-ray photoelectron and emission spectroscopies, as well as electronic structure calculations.
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