Journal
PHYSICAL REVIEW B
Volume 79, Issue 14, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.79.144431
Keywords
critical points; doping profiles; ferromagnetic materials; ferromagnetic-paramagnetic transitions; hydrostatics; magnetic hysteresis; metamagnetism; neodymium compounds; paramagnetic materials; polarons; samarium compounds; strontium compounds
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We report on the magnetic field (H), hydrostatic pressure (P), and doping dependence of the order of the ferromagnetic (FM) to paramagnetic (PM) phase transition in Sm0.52Sr0.48MnO3 single crystal. It has been shown that (H-cr approximate to 4 T, T-cr approximate to 160 K) is a critical point below which FM to PM phase transition is first order in nature accompanied by a sharp drop in resistivity and magnetization with thermal hysteresis. Below the critical point, these parameters also show field-induced metamagnetic transition along with hysteresis between the increasing and decreasing fields. All these signatures of first-order FM transition disappear above the critical point and the transition becomes a crossover. The effect of P on the nature of FM-PM transition is quite similar to that of H and the corresponding critical point, where the character of FM transition that changes from first to second order is (P-cr approximate to 2.5 GPa, T-cr approximate to 160 K). We have also determined the location of critical point expressed in terms of Nd concentration (y) of (Sm1-yNdy)(0.52)Sr0.48MnO3 and found that the transition changes to second order at (y(cr)approximate to 0.4, T-cr approximate to 175 K). The change in the character of FM transition with the application of external (H and P) and internal (Nd concentration) perturbations has been explained within the framework of the formation of polarons.
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