Journal
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 16, Issue 14, Pages 6544-6549Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cp00093e
Keywords
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Funding
- UK EPSRC [EP/C511786/1, EP/F011393]
- ERC [320503 LINASS]
- EU CUBIHOLES
- 3M
- Royal Society
- Wolfson Foundation
- Engineering and Physical Sciences Research Council [EP/K028510/1, EP/C511786/1, EP/G060649/1] Funding Source: researchfish
- EPSRC [EP/K028510/1, EP/G060649/1] Funding Source: UKRI
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The Raman coupling of light to molecular vibrations is strongly modified when they are placed near a plasmonic metal surface, with the appearance of a strong broad continuum background in addition to the normal surface-enhanced Raman scattering (SERS) peaks. Using a quantum method of images approach, we produce a simple but quantitative explanation of the inevitable presence of the background, due to the resistive damping of the image molecule. This model thus suggests new strategies for enhancing the SERS peak to background ratio.
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