Journal
ORGANIC LETTERS
Volume 16, Issue 12, Pages 3316-3319Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol5013263
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Funding
- NIH-NIGMS [R01GM080269]
- Amgen
- Gordon and Betty Moore Foundation
- Caltech
- Fulbright (Foreign Student Program) [15111120]
- Ilju Foundation of Education Culture
- German Academic Exchange Service (DAAD)
- California TRDRP [14FT-0002]
- Bristol-Myers Squibb
- Swiss National Science Foundation
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An efficient, unified, and stereodivergent approach toward communesin F and perophoramidine was examined. The C(3) all-carbon quaternary center of an oxindole was smoothly constructed by base-promoted indolone-malonate alkylation chemistry. The complementary relative stereochemistry of the crucial vicinal quaternary centers found in communesin F and perophoramidine was selectively installed by substrate-controlled decarboxylative allylic alkylations.
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