Journal
ORGANIC LETTERS
Volume 16, Issue 15, Pages 3986-3989Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol501814p
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Funding
- NSFC [21122056, 21372160, 21321061]
- 973 Program [2010CB833300]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT13031]
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A stereoselective inverse-electron-demand aza-Diels-Alder cycloaddition process of cyclic 1-aza-1,3-butadienes and alpha,beta-unsaturated aldehydes has been developed via dienamine catalysis. This reaction exhibits excellent beta,gamma-regioselectivity for enal substrates with substantial structural diversity and broad functionalities, readily producing highly enantioenriched fused piperidine derivatives and enabling efficient sequential construction of complex polycyclic frameworks.
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