Journal
ORGANIC LETTERS
Volume 14, Issue 11, Pages 2914-2917Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol301257m
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Funding
- MEXT [22106523]
- JSPS
- Uehara Memorial Foundation, NOVARTIS Foundation (Japan) for the Promotion of Science
- Takeda Science Foundation
- Grants-in-Aid for Scientific Research [22245006, 20108006, 11J00346, 23655034, 22106523] Funding Source: KAKEN
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Palladium catalysts with bulky biaryl phosphine ligands allow homopropargyl-substituted dicarbonyl compounds to undergo intramolecular addition via a rare 5-endo-dig pathway. C-C bond forming reductive elimination follows the addition to Introduce alkenyl and alkynyl as well as aryl groups by using the corresponding organic halides. The cyclization is versatile enough to be applicable to the synthesis of highly substituted dihydropyrrole and a fused tricyclic compound.
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