Journal
ORGANIC LETTERS
Volume 14, Issue 23, Pages 5940-5943Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol302853m
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Funding
- National Natural Science Foundation of China [21125206, 21021001]
- National Basic Research Program of China (973 Program) [2010CB833300]
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An asymmetric Diels-Alder reaction of 2-methyl-3-indolylmethanols and alpha,beta-unsaturated aldehydes has been developed that relies on in situ generation of active indole-2,3-quinodimethane intermediates under mild acidic conditions and uses a secondary chiral amine as iminium activation catalyst. An array of highly enantioenriched tetrahydrocarbazoles have been efficiently produced in fair to good yields.
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