Journal
ORGANIC LETTERS
Volume 14, Issue 24, Pages 6262-6265Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol303021d
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Funding
- National Research Foundation
- Ministry of Education, Science and Technology [2011-0003298, 2011-0004015]
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A range of tetrahydropyrans and piperidines were produced by Fe(III)-catalyzed intramolecular hydroalkoxylation and hydroamination reactions of allenes. Various Fe catalysts with different counterions were tested. Their activities toward allene and alkene activation depended sensitively on their counterion and reaction conditions. Mechanistic study of the reaction intermediates found a new reaction pattern involving the Fe catalysts and diene substrates.
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