Journal
ORGANIC LETTERS
Volume 13, Issue 18, Pages 4970-4973Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol202129n
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Funding
- Ministerio de Ciencia e Innovacion (MICINN)
- FEDER [CTQ2010-15358, CTQ2009-09949/BQU]
- Junta de Castilla y Leon [BU021A09, GR-172]
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Highly substituted benzene derivatives have been easily prepared in a regioselective way from readily available 1,3-hexadien-5-ynes through a gold(I)-catalyzed tandem reaction. The process involves an initial cyclization followed by a selective Wagner-Meerwein shift in which the migration preference seems to be determined by the ability to stabilize a positive charge.
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