Journal
ORGANIC LETTERS
Volume 12, Issue 3, Pages 544-547Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol902747c
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Funding
- Mitional Natural Science Foundation of China [20872063, 20672057]
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A novel phosphine-mediated reductive cyclopropanation between alpha-substituted allenoates 2 and aldehydes 1 is described. It represents a new member of the allene-based annulations, which provides facile and efficient access to highly functionalized cyclopropanes 3 from simple and readily available starting materials. It also unveils an unprecedented reactivity pattern of allenoates with aldehydes.
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